Low temperature sugar cane bagasse pyrolysis for the production of high purity hydrogen through steam reforming and CO2 capture

被引：9
|
作者：
Lopez Ortiz, A. [1 ]
Neri Segura, F. J. [1 ]
Sandoval Jabalera, R. [2 ]
Marques da Silva Paula, M. [3 ]
Arias del Campo, E. [1 ]
Salinas Gutierrez, J. [1 ]
Escobedo Bretado, M. A. [1 ,4 ]
Collins-Martinez, V. [1 ]
机构：
[1] Ctr Invest Mat Avanzados SC, Dept Mat Nanoestruct, Chihuahua 31109, Chih, Mexico
[2] Univ Autonoma Chihuahua, Fac Ingn, Chihuahua 31240, Chih, Mexico
[3] Univ Extremo Sul Catarinense, PPGCS, Lab Sintese Complexos Multifunc, BR-88806000 Criciuma, Brazil
[4] Univ Juarez Estado Durango, Fac Ciencias Quim, Durango 34120, Dgo, Mexico
来源：
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY | 2013年 / 38卷 / 28期
关键词：
Hydrogen production; Bagasse pyrolysis; Steam reforming; CO2; capture; VACUUM PYROLYSIS; BIOMASS; OIL; DEVOLATILIZATION; ENERGY; YIELD; SLOW; COAL;
D O I：
10.1016/j.ijhydene.2013.06.059
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Biomass pyrolysis offers a fast route to produce elevated yields towards highly valued liquid products. This research aims the determination of optimal experimental conditions for a slow and low temperature pyrolysis to produce the highest yield towards condensable (CVM) and non-condensable (NCVM) volatile matter from Mexican cane bagasse and to quantify and characterize the compounds that constitute CVM and NCVM obtained. Results indicate that yield towards volatiles is strongly dependent on temperature. The highest yield was achieved at temperatures greater than 500 degrees C at a heating rate of 10 degrees C/min, residence time of 60 min and a particle size between of 420 and 840 gm. Product quantification under isothermal conditions determined that at 550 degrees C the NCVM, CVM and solid residue was of 26, 57 and 16%, respectively. Preliminary thermodynamic analysis of steam reforming and CO2 absorption reactions using one of the main CVM products resulted in a potential high hydrogen production yield. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码：12580 / 12588
页数：9
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