Dynamics of polymer translocation into a circular nanocontainer through a nanopore

被引:17
作者
Zhang, Kehong [1 ,2 ]
Luo, Kaifu [1 ]
机构
[1] Univ Sci & Technol China, Dept Polymer Sci & Engn, CAS Key Lab Soft Matter Chem, Hefei 230026, Anhui Province, Peoples R China
[2] Anhui Agr Univ, Coll Light Text Engn & Art, Hefei 230036, Anhui Province, Peoples R China
基金
中国国家自然科学基金;
关键词
DNA TRANSLOCATION; DRIVEN; MOLECULE; SIMULATION; TRANSPORT; MOTION; FORCE;
D O I
10.1063/1.4712618
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Using Langevin dynamics simulations, we investigate the dynamics of polymer translocation into a circular nanocontainer through a nanopore under a driving force F. We observe that the translocation probability initially increases and then saturates with increasing F, independent of phi, which is the average density of the whole chain in the nanocontainer. The translocation time distribution undergoes a transition from a Gaussian distribution to an asymmetric distribution with increasing phi. Moreover, we find a nonuniversal scaling exponent of the translocation time as chain length, depending on phi and F. These results are interpreted by the conformation of the translocated chain in the nanocontainer and the time of an individual segment passing through the pore during translocation. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4712618]
引用
收藏
页数:8
相关论文
共 50 条
[21]   Translocation of a polymer through a nanopore across a viscosity gradient [J].
de Haan, Hendrick W. ;
Slater, Gary W. .
PHYSICAL REVIEW E, 2013, 87 (04)
[22]   Nanoparticle-assisted polymer translocation through a nanopore [J].
Hamidabad, Mohammadreza Niknam ;
Asgari, Sussan ;
Abdolvahab, Rouhollah Haji .
POLYMER, 2020, 204
[23]   Polymer translocation through a nanopore: The effect of solvent conditions [J].
Kapahnke, Felix ;
Schmidt, Ulrich ;
Heermann, Dieter W. ;
Weiss, Matthias .
JOURNAL OF CHEMICAL PHYSICS, 2010, 132 (16)
[24]   Translocation of Copolymers through a Nanopore [J].
Matsuyama, Akihiko ;
Ohno, Kyoko ;
Nishiono, Makoto .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 2013, 82 (02)
[25]   Polymer translocation through nanopore under external electric field: dissipative particle dynamics study [J].
Mao, Jinglin ;
Yao, Yi ;
Zhou, Zhewei ;
Hu, Guohui .
APPLIED MATHEMATICS AND MECHANICS-ENGLISH EDITION, 2015, 36 (12) :1581-1592
[26]   Theory of polymer translocation through a flickering nanopore under an alternating driving force [J].
Sarabadani, Jalal ;
Ikonen, Timo ;
Ala-Nissila, Tapio .
JOURNAL OF CHEMICAL PHYSICS, 2015, 143 (07)
[27]   Using an incremental mean first passage approach to explore the viscosity dependent dynamics of the unbiased translocation of a polymer through a nanopore [J].
de Haan, Hendrick W. ;
Slater, Gary W. .
JOURNAL OF CHEMICAL PHYSICS, 2012, 136 (20)
[28]   Translocation of a polymer through a nanopore starting from a confining nanotube [J].
Sean, David ;
de Haan, Hendrick W. ;
Slater, Gary W. .
ELECTROPHORESIS, 2015, 36 (05) :682-691
[29]   Simulation study on the translocation of a partially charged polymer through a nanopore [J].
Qian, Hong ;
Sun, Li-Zhen ;
Luo, Meng-Bo .
JOURNAL OF CHEMICAL PHYSICS, 2012, 137 (03)
[30]   Driven polymer translocation through a nanopore from a confining channel [J].
Emamyari, Soheila ;
Sarabadani, Jalal ;
Metzler, Ralf ;
Ala-Nissila, Tapio .
JOURNAL OF CHEMICAL PHYSICS, 2025, 162 (24)