Improved performance of solution processed OLEDs using N-annulated perylene diimide emitters with bulky side-chains

被引:27
作者
Dayneko, Sergey V. [1 ,2 ]
Cieplechowicz, Edward [1 ]
Bhojgude, Sachin Suresh [1 ]
Van Humbeck, Jeffrey F. [1 ]
Pahlevani, Majid [3 ]
Welch, Gregory C. [1 ]
机构
[1] Univ Calgary, Dept Chem, 731Campus Pl NW, Calgary, AB T2N 1N4, Canada
[2] Genoptic LED Inc, 6000 72nd Ave SE, Calgary, AB T2C 5C3, Canada
[3] Queens Univ, Dept Elect & Comp Engn, 19 Union St, Kingston, ON K7L 3N6, Canada
来源
MATERIALS ADVANCES | 2021年 / 2卷 / 03期
关键词
LIGHT-EMITTING-DIODES; 3,4,9,10-PERYLENETETRACARBOXYLIC DIANHYDRIDE DYES; EFFICIENCY; RED; PHOTOCHEMISTRY; ABSORPTION; PROGRESS;
D O I
10.1039/d0ma00827c
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We have designed and synthesized three N-annulated perylene diimide (PDI) compounds containing sterically bulky alkyl-substituted benzyl moieties (PDI-X, where X = 1, 2, 3) with photoluminescence quantum yield (PLQY) in the solid-state >20%. The PDI molecules show PLQY of similar to 0.8 in solution and similar to 0.2 as neat films. Organic light-emitting diodes (OLEDs) have been fabricated using these new PDI molecules as light emitters with the active layer being solution processed from non-halogenated solvents. The OLED devices had brightness of similar to 2000 cd m(-2) and low turn-on voltage of similar to 3 V, among the best for PDI based red colored OLEDs.
引用
收藏
页码:933 / 936
页数:4
相关论文
共 38 条
[1]   Device efficiency of organic light-emitting diodes: Progress by improved light outcoupling [J].
Bruetting, Wolfgang ;
Frischeisen, Joerg ;
Schmidt, Tobias D. ;
Scholz, Bert J. ;
Mayr, Christian .
PHYSICA STATUS SOLIDI A-APPLICATIONS AND MATERIALS SCIENCE, 2013, 210 (01) :44-65
[2]   N-Annulated perylene diimide dimers: acetylene linkers as a strategy for controlling structural conformation and the impact on physical, electronic, optical and photovoltaic properties [J].
Cann, Jonathan ;
Dayneko, Sergey ;
Sun, Jon-Paul ;
Hendsbee, Arthur D. ;
Hill, Ian G. ;
Welch, Gregory C. .
JOURNAL OF MATERIALS CHEMISTRY C, 2017, 5 (08) :2074-2083
[3]   Solution processed red organic light-emitting-diodes using an N-annulated perylene diimide fluorophore [J].
Dayneko, Sergey V. ;
Rahmati, Mohammad ;
Pahlevani, Majid ;
Welch, Gregory C. .
JOURNAL OF MATERIALS CHEMISTRY C, 2020, 8 (07) :2314-2319
[4]   Ternary organic solar cells: using molecular donor or acceptor third components to increase open circuit voltage [J].
Dayneko, Sergey, V ;
Hendsbee, Arthur D. ;
Cann, Jonathan R. ;
Cabanetos, Clement ;
Welch, Gregory C. .
NEW JOURNAL OF CHEMISTRY, 2019, 43 (26) :10442-10448
[5]   Combining Facile Synthetic Methods with Greener Processing for Efficient Polymer-Perylene Diimide Based Organic Solar Cells [J].
Dayneko, Sergey V. ;
Hendsbee, Arthur D. ;
Welch, Gregory C. .
SMALL METHODS, 2018, 2 (06)
[6]   Fullerene-free polymer solar cells processed from non-halogenated solvents in air with PCE of 4.8% [J].
Dayneko, Sergey V. ;
Hendsbee, Arthur D. ;
Welch, Gregory C. .
CHEMICAL COMMUNICATIONS, 2017, 53 (06) :1164-1167
[8]   PHOTOCHEMISTRY OF 3,4,9,10-PERYLENETETRACARBOXYLIC DIANHYDRIDE DYES .3. SINGLET AND TRIPLET EXCITED-STATE PROPERTIES OF THE BIS(2,5-DI-TERT-BUTYLPHENYL)IMIDE DERIVATIVE [J].
FORD, WE ;
KAMAT, PV .
JOURNAL OF PHYSICAL CHEMISTRY, 1987, 91 (25) :6373-6380
[9]   Organic light-emitting diode (OLED) technology: materials, devices and display technologies [J].
Geffroy, Bernard ;
le Roy, Philippe ;
Prat, Christophe .
POLYMER INTERNATIONAL, 2006, 55 (06) :572-582
[10]   ANGULAR-DEPENDENCE OF THE EMISSION FROM A CONJUGATED POLYMER LIGHT-EMITTING DIODE - IMPLICATIONS FOR EFFICIENCY CALCULATIONS [J].
GREENHAM, NC ;
FRIEND, RH ;
BRADLEY, DDC .
ADVANCED MATERIALS, 1994, 6 (06) :491-494