Optical emission from a charge-tunable quantum ring

被引:822
作者
Warburton, RJ
Schäflein, C
Haft, D
Bickel, F
Lorke, A
Karrai, K
Garcia, JM
Schoenfeld, W
Petroff, PM
机构
[1] Univ Munich, Sekt Phys, D-80539 Munich, Germany
[2] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA
[3] Univ Calif Santa Barbara, QUEST, Santa Barbara, CA 93106 USA
[4] Univ Munich, Ctr Nanosci, D-80539 Munich, Germany
关键词
D O I
10.1038/35016030
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Quantum dots or rings are artificial nanometre-sized clusters that confine electrons in all three directions. They can be fabricated in a semiconductor system by embedding an island of low-bandgap material in a sea of material with a higher bandgap. Quantum dots are often referred to as artificial atoms because, when filled sequentially with electrons, the charging energies are pronounced for particular electron numbers(1-3); this is analogous to Hund's rules in atomic physics. But semiconductors also have a valence band with strong optical transitions to the conduction band. These transitions are the basis for the application of quantum dots as laser emitters(4), storage devices(5-7) and fluorescence markers(8). Here we report how the optical emission (photoluminescence) of a single quantum ring changes as electrons are added one-by-one. We find that the emission energy changes abruptly whenever an electron is added to the artificial atom, and that the sizes of the jumps reveal a shell structure.
引用
收藏
页码:926 / 929
页数:5
相关论文
共 24 条
[1]  
[Anonymous], QUANTUM DOT HETEROST
[2]   N-ELECTRON GROUND-STATE ENERGIES OF A QUANTUM-DOT IN MAGNETIC-FIELD [J].
ASHOORI, RC ;
STORMER, HL ;
WEINER, JS ;
PFEIFFER, LN ;
BALDWIN, KW ;
WEST, KW .
PHYSICAL REVIEW LETTERS, 1993, 71 (04) :613-616
[3]   Identification of atomic-like electronic states in indium arsenide nanocrystal quantum dots [J].
Banin, U ;
Cao, YW ;
Katz, D ;
Millo, O .
NATURE, 1999, 400 (6744) :542-544
[4]   Electron and hole g factors and exchange interaction from studies of the exciton fine structure in In0.60Ga0.40As quantum dots [J].
Bayer, M ;
Kuther, A ;
Forchel, A ;
Gorbunov, A ;
Timofeev, VB ;
Schäfer, F ;
Reithmaier, JP ;
Reinecke, TL ;
Walck, SN .
PHYSICAL REVIEW LETTERS, 1999, 82 (08) :1748-1751
[5]   EXCHANGE INTERACTION OF EXCITONS IN GAAS HETEROSTRUCTURES [J].
BLACKWOOD, E ;
SNELLING, MJ ;
HARLEY, RT ;
ANDREWS, SR ;
FOXON, CTB .
PHYSICAL REVIEW B, 1994, 50 (19) :14246-14254
[6]   Time resolved spectroscopy of single quantum dots: Fermi gas of excitons? [J].
Bockelmann, U ;
Roussignol, P ;
Filoramo, A ;
Heller, W ;
Abstreiter, G ;
Brunner, K ;
Bohm, G ;
Weimann, G .
PHYSICAL REVIEW LETTERS, 1996, 76 (19) :3622-3625
[7]   Semiconductor nanocrystals as fluorescent biological labels [J].
Bruchez, M ;
Moronne, M ;
Gin, P ;
Weiss, S ;
Alivisatos, AP .
SCIENCE, 1998, 281 (5385) :2013-2016
[8]   Multiexciton spectroscopy of a single self-assembled quantum dot [J].
Dekel, E ;
Gershoni, D ;
Ehrenfreund, E ;
Spektor, D ;
Garcia, JM ;
Petroff, PM .
PHYSICAL REVIEW LETTERS, 1998, 80 (22) :4991-4994
[9]   SPECTROSCOPY OF QUANTUM LEVELS IN CHARGE-TUNABLE INGAAS QUANTUM DOTS [J].
DREXLER, H ;
LEONARD, D ;
HANSEN, W ;
KOTTHAUS, JP ;
PETROFF, PM .
PHYSICAL REVIEW LETTERS, 1994, 73 (16) :2252-2255
[10]   Quantum-confined stark effect in single CdSe nanocrystallite quantum dots [J].
Empedocles, SA ;
Bawendi, MG .
SCIENCE, 1997, 278 (5346) :2114-2117