Concentration variability of anthropogenic halocarbons and applications as internal reference in volatile organic compound measurements

被引:30
作者
Wang, JL [1 ]
Chew, C [1 ]
Chen, SW [1 ]
Kuo, SR [1 ]
机构
[1] Natl Cent Univ, Dept Chem, Chungli 320, Taiwan
关键词
D O I
10.1021/es991128n
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This work investigated concentration variability of anthropogenic halocarbons by performing four separate sample collections in urban, industrial, and back-ground atmospheric environments. Large concentration variability was found for CFC-12, CH3CCl3, CClH=CCl2, and CCl2=CCl2 in nonbackground environments. in comparison, the variability of CFC-113 and CCl4 was small regardless of the environments and was also close to the precision of the analytical system, implying that CFC-113 and CCl4 have relatively little emissions in Taiwan. The uniform property associated with atmospheric CCl4 is suggested as an "intrinsic" internal reference for quality control of VOC analysis.
引用
收藏
页码:2243 / 2248
页数:6
相关论文
共 33 条
[1]  
[Anonymous], TO1 US EPA
[2]  
[Anonymous], 1987, MONTR PROT SUBST DEP
[3]   SUMMERTIME MEASUREMENTS OF SELECTED NONMETHANE HYDROCARBONS IN THE ARCTIC AND SUB-ARCTIC DURING THE 1988 ARCTIC BOUNDARY-LAYER EXPEDITION (ABLE-3A) [J].
BLAKE, DR ;
HURST, DF ;
SMITH, TW ;
WHIPPLE, WJ ;
CHEN, TY ;
BLAKE, NJ ;
ROWLAND, FS .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1992, 97 (D15) :16559-16588
[4]   GLOBAL ATMOSPHERIC CONCENTRATIONS AND SOURCE STRENGTH OF ETHANE [J].
BLAKE, DR ;
ROWLAND, FS .
NATURE, 1986, 321 (6067) :231-233
[5]   A DETAILED MECHANISM FOR THE GAS-PHASE ATMOSPHERIC REACTIONS OF ORGANIC-COMPOUNDS [J].
CARTER, WPL .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1990, 24 (03) :481-518
[6]   Estimation of global vehicular methyl bromide emissions: Extrapolation from a case study in Santiago, Chile [J].
Chen, TY ;
Blake, DR ;
Lopez, JP ;
Rowland, FS .
GEOPHYSICAL RESEARCH LETTERS, 1999, 26 (03) :283-286
[7]   GLOBAL TRENDS AND ANNUAL RELEASES OF CCL3F AND CCL2F2 ESTIMATED FROM ALE/GAGE AND OTHER MEASUREMENTS FROM JULY 1978 TO JUNE 1991 [J].
CUNNOLD, DM ;
FRASER, PJ ;
WEISS, RF ;
PRINN, RG ;
SIMMONDS, PG ;
MILLER, BR ;
ALYEA, FN ;
CRAWFORD, AJ .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1994, 99 (D1) :1107-1126
[8]   GAGE/AGAGE measurements indicating reductions in global emissions of CCl3F and CCl2F2 in 1992-1994 [J].
Cunnold, DM ;
Weiss, RF ;
Prinn, RG ;
Hartley, D ;
Simmonds, PG ;
Fraser, PJ ;
Miller, B ;
Alyea, FN ;
Porter, L .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1997, 102 (D1) :1259-1269
[9]   DIRECT CHROMATOGRAPHIC COMPARISON OF THE RELATIVE ADSORPTION ACTIVITY OF VARIOUS TYPES OF CAPILLARY TRANSFER TUBING [J].
DALLAS, AJ ;
CARR, PW .
ANALYTICA CHIMICA ACTA, 1991, 251 (1-2) :83-93
[10]   DECREASE IN THE GROWTH-RATES OF ATMOSPHERIC CHLOROFLUOROCARBON-11 AND CHLOROFLUOROCARBON-12 [J].
ELKINS, JW ;
THOMPSON, TM ;
SWANSON, TH ;
BUTLER, JH ;
HALL, BD ;
CUMMINGS, SO ;
FISHER, DA ;
RAFFO, AG .
NATURE, 1993, 364 (6440) :780-783