Isotopic signatures of mercury contamination in latest Permian oceans

被引:225
作者
Grasby, Stephen E. [1 ,2 ]
Shen, Wenjie [3 ]
Yin, Runsheng [4 ,5 ]
Gleason, James D. [6 ]
Blum, Joel D. [6 ]
Lepak, Ryan F. [5 ]
Hurley, James P. [5 ]
Beauchamp, Benoit [2 ]
机构
[1] Nat Resources Canada, Geol Survey Canada, 3303 33rd St NW, Calgary, AB T2L 2A7, Canada
[2] Univ Calgary, Dept Geosci, 2500 Univ Dr NW, Calgary, AB T2N 1N4, Canada
[3] Sun Yat Sen Univ, Sch Earth Sci & Geol Engn, Guangzhou 510275, Guangdong, Peoples R China
[4] Chinese Acad Sci, Inst Geochem, State Key Lab Ore Deposit Geochem, Guiyang 550002, Peoples R China
[5] Univ Wisconsin, Environm Chem & Technol Program, Madison, WI 53706 USA
[6] Univ Michigan, Dept Earth & Environm Sci, Ann Arbor, MI 48109 USA
基金
美国国家科学基金会;
关键词
ATMOSPHERIC HG; DEPOSITION; SECTION;
D O I
10.1130/G38487.1
中图分类号
P5 [地质学];
学科分类号
0709 ; 081803 ;
摘要
Sedimentary records from the northwest margin of Pangea and the Tethys show anomalously high Hg levels at the latest Permian extinction boundary. Background delta Hg-202 values are consistent with normal marine conditions but exhibit negative shifts coincident with increased Hg concentrations. Hg isotope mass-independent fractionation (Delta Hg-199) trends are consistent with volcanic input in deep-water marine environments. In contrast, nearshore environments have Delta Hg-199 signatures consistent with enhanced soil and/or biomass input. We hypothesize that the deep-water signature represents an overall global increase in volcanic Hg input and that this isotope signature is overwhelmed in nearshore locations due to Hg from terrestrial sources. High-productivity nearshore regions may have experienced stressed marine ecosystems due to enhanced Hg loading.
引用
收藏
页码:55 / 58
页数:4
相关论文
共 33 条
[1]   Anomalous Early Triassic sediment fluxes due to elevated weathering rates and their biological consequences [J].
Algeo, Thomas J. ;
Twitchett, Richard J. .
GEOLOGY, 2010, 38 (11) :1023-1026
[2]  
[Anonymous], 2010, ATMOS CHEM PHYS, DOI DOI 10.5194/ACPD-10-4719-2010
[3]   Impacts of global warming on Permo-Triassic terrestrial ecosystems [J].
Benton, Michael J. ;
Newell, Andrew J. .
GONDWANA RESEARCH, 2014, 25 (04) :1308-1337
[4]   Mass-dependent and -independent fractionation of Hg isotopes by photoreduction in aquatic systems [J].
Bergquist, Bridget A. ;
Blum, Joel D. .
SCIENCE, 2007, 318 (5849) :417-420
[5]   Mercury Isotopes in Earth and Environmental Sciences [J].
Blum, Joel D. ;
Sherman, Laura S. ;
Johnson, Marcus W. .
ANNUAL REVIEW OF EARTH AND PLANETARY SCIENCES, VOL 42, 2014, 42 :249-269
[6]   High-precision geochronology confirms voluminous magmatism before, during, and after Earth's most severe extinction [J].
Burgess, Seth D. ;
Bowring, Samuel A. .
SCIENCE ADVANCES, 2015, 1 (07)
[7]   Odd Isotope Deficits in Atmospheric Hg Measured in Lichens [J].
Carignan, Jean ;
Estrade, Nicolas ;
Sonke, Jeroen E. ;
Donard, Olivier F. X. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2009, 43 (15) :5660-5664
[8]   A comparison of Eastern Boundary Upwelling Ecosystems [J].
Chavez, Francisco P. ;
Messie, Monique .
PROGRESS IN OCEANOGRAPHY, 2009, 83 (1-4) :80-96
[9]  
Chen ZQ, 2012, NAT GEOSCI, V5, P375, DOI [10.1038/ngeo1475, 10.1038/NGEO1475]
[10]   Mercury isotopes in a forested ecosystem: Implications for air-surface exchange dynamics and the global mercury cycle [J].
Demers, Jason D. ;
Blum, Joel D. ;
Zak, Donald R. .
GLOBAL BIOGEOCHEMICAL CYCLES, 2013, 27 (01) :222-238