The Rational Design of a Single-Component Photocatalyst for Gas-Phase CO2 Reduction Using Both UV and Visible Light

被引：212

作者：

Hoch, Laura B. ^{[1
]}

Wood, Thomas E. ^{[2
]}

O'Brien, Paul G. ^{[1
]}

Liao, Kristine ^{[1
]}

Reyes, Laura M. ^{[1
]}

Mims, Charles A. ^{[2
]}

Ozin, Geoffrey A. ^{[1
]}

机构：

[1] Univ Toronto, Dept Chem, Mat Chem Res Grp, 80 St George St, Toronto, ON M5S 3H6, Canada

[2] Univ Toronto, Dept Chem Engn & Appl Chem, Toronto, ON M5S 3E5, Canada

来源：

ADVANCED SCIENCE | 2014年 / 1卷 / 01期

基金：

加拿大自然科学与工程研究理事会;

关键词：

ARTIFICIAL PHOTOSYNTHESIS; OXYGEN VACANCY; CARBON-DIOXIDE; TIO2; SEMICONDUCTORS; PHOTOREDUCTION; HYDROGENATION; CATALYSTS; VALENCE;

D O I：

10.1002/advs.201400013

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The solar-to-chemical energy conversion of greenhouse gas CO2 into carbon-based fuels is a very important research challenge, with implications for both climate change and energy security. Herein, the key attributes of hydroxides and oxygen vacancies are experimentally identified in non-stoichiometric indium oxide nanoparticles, In2O3-x(OH)y, that function in concert to reduce CO2 to CO under simulated solar irradiation. © 2014 The Authors.

引用

页数：10

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