A novel tellurophene-containing conjugated polymer with a dithiophenyl diketopyrrolopyrrole unit for use in organic thin film transistors

被引:73
作者
Kaur, Matinder [1 ]
Yang, Da Seul [1 ]
Shin, Jicheol [1 ]
Lee, Tae Wan [1 ]
Choi, Kihang [1 ]
Cho, Min Ju [1 ]
Choi, Dong Hoon [1 ]
机构
[1] Korea Univ, Res Inst Nat Sci, Dept Chem, Seoul 136701, South Korea
基金
新加坡国家研究基金会;
关键词
FIELD-EFFECT TRANSISTORS; ALKYL SIDE-CHAINS; COPOLYMERS; SEMICONDUCTORS; MOBILITY;
D O I
10.1039/c3cc41250d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A new tellurophene-based pi-conjugated polymer, PDTDPPTe, was synthesized. PDTDPPTe exhibits a smaller optical band gap (E-g(opt) = 1.25 eV) than thiophene-based PDTDPPT (E-g(opt) = 1.30 eV). Thin-film transistors comprising PDTDPPTe displayed outstanding performance (mu(max) = 1.78 cm(2) V-1 s(-1), I-on/I-off = 10(5-6)).
引用
收藏
页码:5495 / 5497
页数:3
相关论文
共 33 条
[21]   Conjugated polymer-based chemical sensors [J].
McQuade, DT ;
Pullen, AE ;
Swager, TM .
CHEMICAL REVIEWS, 2000, 100 (07) :2537-2574
[22]   Electronic and molecular structures of polyheteroles: II. Aromaticity and quinoidicity [J].
Narita, Y ;
Takeda, K .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 2006, 45 (4A) :2628-2642
[23]   Polyselenophenes [J].
Patra, Asit ;
Bendikov, Michael .
JOURNAL OF MATERIALS CHEMISTRY, 2010, 20 (03) :422-433
[24]   Tuning the Band Gap of Low-Band-Gap Polyselenophenes and Polythiophenes: The Effect of the Heteroatom [J].
Patra, Asit ;
Wijsboom, Yair H. ;
Leitus, Gregory ;
Bendikov, Michael .
CHEMISTRY OF MATERIALS, 2011, 23 (03) :896-906
[25]   Synthesis, Structure, and Electropolymerization of 3,4-Dimethoxytellurophene: Comparison with Selenium Analogue [J].
Patra, Asit ;
Wijsboom, Yair H. ;
Leitus, Gregory ;
Bendikov, Michael .
ORGANIC LETTERS, 2009, 11 (07) :1487-1490
[26]   CONJUGATED POLY(THIOPHENES) - SYNTHESIS, FUNCTIONALIZATION, AND APPLICATIONS [J].
RONCALI, J .
CHEMICAL REVIEWS, 1992, 92 (04) :711-738
[27]   Photovoltaic and field effect transistor performance of selenophene and thiophene diketopyrrolopyrrole co-polymers with dithienothiophene [J].
Shahid, Munazza ;
Ashraf, Raja Shahid ;
Huang, Zhenggang ;
Kronemeijer, Auke J. ;
McCarthy-Ward, Thomas ;
McCulloch, Iain ;
Durrant, James R. ;
Sirringhaus, Henning ;
Heeney, Martin .
JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (25) :12817-12823
[28]   Telluranes:: potential synthons for charge-transfer complexes (involving hypervalent Te-I bonds) and serendipitous synthesis of the first triphenyl methyl phosphonium salts containing [C4H8TeI4]2- and [TeI6]2-anions [J].
Srivastava, PC ;
Bajpai, S ;
Bajpai, S ;
Ram, C ;
Kumar, R ;
Jasinski, JP ;
Butcher, RJ .
JOURNAL OF ORGANOMETALLIC CHEMISTRY, 2004, 689 (01) :194-202
[29]   Synthesis and Stille Cross-Coupling Reactions of 2-(Tributylstannyl)- and 2,5-Bis(trimethylstannyl)tellurophene [J].
Sweat, Daniel P. ;
Stephens, Chad E. .
SYNTHESIS-STUTTGART, 2009, (19) :3214-3218
[30]   Conjugated polymers containing diketopyrrolopyrrole units in the main chain [J].
Tieke, Bernd ;
Rabindranath, A. Raman ;
Zhang, Kai ;
Zhu, Yu .
BEILSTEIN JOURNAL OF ORGANIC CHEMISTRY, 2010, 6 :830-845