A novel tellurophene-containing conjugated polymer with a dithiophenyl diketopyrrolopyrrole unit for use in organic thin film transistors

被引:70
作者
Kaur, Matinder [1 ]
Yang, Da Seul [1 ]
Shin, Jicheol [1 ]
Lee, Tae Wan [1 ]
Choi, Kihang [1 ]
Cho, Min Ju [1 ]
Choi, Dong Hoon [1 ]
机构
[1] Korea Univ, Res Inst Nat Sci, Dept Chem, Seoul 136701, South Korea
基金
新加坡国家研究基金会;
关键词
FIELD-EFFECT TRANSISTORS; ALKYL SIDE-CHAINS; COPOLYMERS; SEMICONDUCTORS; MOBILITY;
D O I
10.1039/c3cc41250d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A new tellurophene-based pi-conjugated polymer, PDTDPPTe, was synthesized. PDTDPPTe exhibits a smaller optical band gap (E-g(opt) = 1.25 eV) than thiophene-based PDTDPPT (E-g(opt) = 1.30 eV). Thin-film transistors comprising PDTDPPTe displayed outstanding performance (mu(max) = 1.78 cm(2) V-1 s(-1), I-on/I-off = 10(5-6)).
引用
收藏
页码:5495 / 5497
页数:3
相关论文
共 33 条
  • [21] Conjugated polymer-based chemical sensors
    McQuade, DT
    Pullen, AE
    Swager, TM
    [J]. CHEMICAL REVIEWS, 2000, 100 (07) : 2537 - 2574
  • [22] Electronic and molecular structures of polyheteroles: II. Aromaticity and quinoidicity
    Narita, Y
    Takeda, K
    [J]. JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 2006, 45 (4A): : 2628 - 2642
  • [23] Polyselenophenes
    Patra, Asit
    Bendikov, Michael
    [J]. JOURNAL OF MATERIALS CHEMISTRY, 2010, 20 (03) : 422 - 433
  • [24] Tuning the Band Gap of Low-Band-Gap Polyselenophenes and Polythiophenes: The Effect of the Heteroatom
    Patra, Asit
    Wijsboom, Yair H.
    Leitus, Gregory
    Bendikov, Michael
    [J]. CHEMISTRY OF MATERIALS, 2011, 23 (03) : 896 - 906
  • [25] Synthesis, Structure, and Electropolymerization of 3,4-Dimethoxytellurophene: Comparison with Selenium Analogue
    Patra, Asit
    Wijsboom, Yair H.
    Leitus, Gregory
    Bendikov, Michael
    [J]. ORGANIC LETTERS, 2009, 11 (07) : 1487 - 1490
  • [26] CONJUGATED POLY(THIOPHENES) - SYNTHESIS, FUNCTIONALIZATION, AND APPLICATIONS
    RONCALI, J
    [J]. CHEMICAL REVIEWS, 1992, 92 (04) : 711 - 738
  • [27] Photovoltaic and field effect transistor performance of selenophene and thiophene diketopyrrolopyrrole co-polymers with dithienothiophene
    Shahid, Munazza
    Ashraf, Raja Shahid
    Huang, Zhenggang
    Kronemeijer, Auke J.
    McCarthy-Ward, Thomas
    McCulloch, Iain
    Durrant, James R.
    Sirringhaus, Henning
    Heeney, Martin
    [J]. JOURNAL OF MATERIALS CHEMISTRY, 2012, 22 (25) : 12817 - 12823
  • [28] Telluranes:: potential synthons for charge-transfer complexes (involving hypervalent Te-I bonds) and serendipitous synthesis of the first triphenyl methyl phosphonium salts containing [C4H8TeI4]2- and [TeI6]2-anions
    Srivastava, PC
    Bajpai, S
    Bajpai, S
    Ram, C
    Kumar, R
    Jasinski, JP
    Butcher, RJ
    [J]. JOURNAL OF ORGANOMETALLIC CHEMISTRY, 2004, 689 (01) : 194 - 202
  • [29] Synthesis and Stille Cross-Coupling Reactions of 2-(Tributylstannyl)- and 2,5-Bis(trimethylstannyl)tellurophene
    Sweat, Daniel P.
    Stephens, Chad E.
    [J]. SYNTHESIS-STUTTGART, 2009, (19): : 3214 - 3218
  • [30] Conjugated polymers containing diketopyrrolopyrrole units in the main chain
    Tieke, Bernd
    Rabindranath, A. Raman
    Zhang, Kai
    Zhu, Yu
    [J]. BEILSTEIN JOURNAL OF ORGANIC CHEMISTRY, 2010, 6 : 830 - 845