A novel tellurophene-containing conjugated polymer with a dithiophenyl diketopyrrolopyrrole unit for use in organic thin film transistors

被引：70

作者：

Kaur, Matinder ^{[1
]}

Yang, Da Seul ^{[1
]}

Shin, Jicheol ^{[1
]}

Lee, Tae Wan ^{[1
]}

Choi, Kihang ^{[1
]}

Cho, Min Ju ^{[1
]}

Choi, Dong Hoon ^{[1
]}

机构：

[1] Korea Univ, Res Inst Nat Sci, Dept Chem, Seoul 136701, South Korea

来源：

CHEMICAL COMMUNICATIONS | 2013年 / 49卷 / 48期

基金：

新加坡国家研究基金会;

关键词：

FIELD-EFFECT TRANSISTORS; ALKYL SIDE-CHAINS; COPOLYMERS; SEMICONDUCTORS; MOBILITY;

D O I：

10.1039/c3cc41250d

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A new tellurophene-based pi-conjugated polymer, PDTDPPTe, was synthesized. PDTDPPTe exhibits a smaller optical band gap (E-g(opt) = 1.25 eV) than thiophene-based PDTDPPT (E-g(opt) = 1.30 eV). Thin-film transistors comprising PDTDPPTe displayed outstanding performance (mu(max) = 1.78 cm(2) V-1 s(-1), I-on/I-off = 10(5-6)).

引用

页码：5495 / 5497

页数：3

共 33 条

[1] Organic semiconductors for solution-processable field-effect transistors (OFETs)
Allard, Sybille
Forster, Michael
Souharce, Benjamin
Thiem, Heiko
Scherf, Ullrich
[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (22) : 4070 - 4098
[2] Te-Te interactions in inorganic rings with sulfur donors
Bandeira, NAG
Veiros, LF
Calhorda, MJ
Novosad, J
[J]. INORGANICA CHIMICA ACTA, 2003, 356 : 319 - 327
[3] CONVENIENT SYNTHESIS OF TELLUROPHENE
BARTON, TJ
ROTH, RW
[J]. JOURNAL OF ORGANOMETALLIC CHEMISTRY, 1972, 39 (02) : C66 - &
[4] Impact of the Alkyl Side Chains on the Optoelectronic Properties of a Series of Photovoltaic Low-Band-Gap Copolymers
Biniek, Laure
Fall, Sadiara
Chochos, Christos L.
Anokhin, Denis V.
Ivanov, Dimitri A.
Leclerc, Nicolas
Leveque, Patrick
Heiser, Thomas
[J]. MACROMOLECULES, 2010, 43 (23) : 9779 - 9786
[5] Synthesis of Conjugated Polymers for Organic Solar Cell Applications
Cheng, Yen-Ju
Yang, Sheng-Hsiung
Hsu, Chain-Shu
[J]. CHEMICAL REVIEWS, 2009, 109 (11) : 5868 - 5923
[6] Influence of heteroaryl group on electrochemical and spectroscopic properties of conjugated polymers
Data, P.
Lapkowski, M.
Motyka, R.
Suwinski, J.
[J]. ELECTROCHIMICA ACTA, 2012, 83 : 271 - 282
[7] Devillanova FA, 2007, HANDBOOK OF CHALCOGEN CHEMISTRY: NEW PERSPECTIVES IN SULFUR, SELENIUM AND TELLURIUM, P1, DOI 10.1039/9781847557575
[8] Electroluminescent materials for white organic light emitting diodes
Farinola, Gianluca M.
Ragni, Roberta
[J]. CHEMICAL SOCIETY REVIEWS, 2011, 40 (07) : 3467 - 3482
[9] Fichou D., 1999, Handbook of Oligo- and Polythiophenes
[10] Atomistic Band Gap Engineering in Donor-Acceptor Polymers
Gibson, Gregory L.
McCormick, Theresa M.
Seferos, Dwight S.
[J]. JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (01) : 539 - 547

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