Update on mixed-salt technology development for CO2 capture from post-combustion power stations

被引:15
作者
Jayaweera, Indira [1 ]
Jayaweera, Palitha [1 ]
Elmore, Regina [1 ]
Bao, Jianer [1 ]
Bhamidi, Srinivas [1 ]
机构
[1] SRI Int, Menlo Pk, CA 94025 USA
来源
12TH INTERNATIONAL CONFERENCE ON GREENHOUSE GAS CONTROL TECHNOLOGIES, GHGT-12 | 2014年 / 63卷
关键词
CO2; capture; post-combustion; mixed-salt; ammonia; potasium carbonate;
D O I
10.1016/j.egypro.2014.11.070
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
The new mixed-salt technology combines the well-known ammonia and potassium carbonate technologies with improved reaction kinetics and reduced emissions. This technology is capable of capturing CO2 at high cyclic loadings compared to amine-based processes. In addition, mixed-salt technology can strip CO2 at high pressure, reducing the CO2 compression costs, requires no solvent chilling as in aqueous ammonia based processes, and has a low reboiler duty for regeneration (< 1000 Btu/lb.). Mixed-salt technology provides unique opportunities for better energy management to reduce the burden on the power plant steam cycle and is suitable for capturing CO2 from post-combustion, pre-combustion and other industrial gas streams. The mixed-salt technology has already been tested successfully in two small bench-level systems and is currently being tested at a large bench-scale pilot level with the funding from the U.S. Department of Energy (DOE). The technology can easily be scaled up with use of conventional process equipment and can be demonstrated in full scale sooner than second-generation technologies that are currently in development. (C) 2014 The Authors. Published by Elsevier Ltd.
引用
收藏
页码:640 / 650
页数:11
相关论文
共 12 条
[1]   CO2 capture from power plants.: Part I.: A parametric study of the technical-performance based on monoethanolamine [J].
Abu-Zahra, Mohammad R. M. ;
Schneiders, Leon H. J. ;
Niederer, John P. M. ;
Feron, Paul H. M. ;
Versteeg, Geert F. .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2007, 1 (01) :37-46
[2]  
[Anonymous], 2012, GET CARB CAPT STOR C
[3]  
Cullinane J. T., 2005, DEFC2602NT41440 DOE
[4]  
Gal E., 2011, U. S. Patent, Patent No. [7,846,240, 7846240]
[5]  
Jayaweera, 2013, PREPR PAP AM CHEM SO, V58, P58
[6]  
Kalicki Jan H., 2013, ENERGY SECURITY STRA
[7]  
Kothandaraman A, 2010, THESIS MIT
[8]   New Amines for CO2 Capture. IV. Degradation, Corrosion, and Quantitative Structure Property Relationship Model [J].
Martin, Sandrine ;
Lepaumier, Helene ;
Picq, Dominique ;
Kittel, Jean ;
de Bruin, Theodorus ;
Faraj, Abdelaziz ;
Carrette, Pierre-Louis .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2012, 51 (18) :6283-6289
[9]   Techno-economic analysis of natural gas combined cycles with post-combustion CO2 absorption, including a detailed evaluation of the development potential [J].
Peeters, A. N. M. ;
Faaij, A. P. C. ;
Turkenburg, W. C. .
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2007, 1 (04) :396-417
[10]   Amine Scrubbing for CO2 Capture [J].
Rochelle, Gary T. .
SCIENCE, 2009, 325 (5948) :1652-1654