NMR evidence for spin fluctuations in the bilayer nickelate La3Ni2O6

被引:10
作者
ApRoberts-Warren, N. [1 ]
Crocker, J. [1 ]
Dioguardi, A. P. [1 ]
Shirer, K. R. [1 ]
Poltavets, V. V. [2 ]
Greenblatt, M. [3 ]
Klavins, P. [1 ]
Curro, N. J. [1 ]
机构
[1] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA
[2] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA
[3] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevB.88.075124
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report nuclear magnetic resonance data in the bilayer nickelate La3Ni2O6. This material belongs to a family of low valence nickel oxides with square planar coordination of the Ni ions and is isoelectronic to the high temperature superconducting cuprates. Although the three layer nickelate compound exhibits a spin-state transition accompanied by antiferromagnetic order, the bilayer material shows no phase transition. The NMR data in the bilayer La3Ni2O6 reveal the presence of antiferromagnetic spin fluctuations down to 5K that are surprisingly similar to those present in the magnetically ordered trilayer La4Ni3O8, suggesting a similar electronic structure in the paramagnetic phase of both compounds.
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页数:5
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共 17 条
[1]   Electronic structure of possible nickelate analogs to the cuprates [J].
Anisimov, VI ;
Bukhvalov, D ;
Rice, TM .
PHYSICAL REVIEW B, 1999, 59 (12) :7901-7906
[2]   Critical spin dynamics in the antiferromagnet La4Ni3O8 from 139La nuclear magnetic resonance [J].
ApRoberts-Warren, Nicholas ;
Dioguardi, Adam P. ;
Poltavets, Viktor V. ;
Greenblatt, Martha ;
Klavins, Peter ;
Curro, Nicholas J. .
PHYSICAL REVIEW B, 2011, 83 (01)
[3]   Dimensionality Control of Electronic Phase Transitions in Nickel-Oxide Superlattices [J].
Boris, A. V. ;
Matiks, Y. ;
Benckiser, E. ;
Frano, A. ;
Popovich, P. ;
Hinkov, V. ;
Wochner, P. ;
Castro-Colin, M. ;
Detemple, E. ;
Malik, V. K. ;
Bernhard, C. ;
Prokscha, T. ;
Suter, A. ;
Salman, Z. ;
Morenzoni, E. ;
Cristiani, G. ;
Habermeier, H. -U. ;
Keimer, B. .
SCIENCE, 2011, 332 (6032) :937-940
[4]   Pressure Effect on the Structural Transition and Suppression of the High-Spin State in the Triple-Layer T′-La4Ni3O8 [J].
Cheng, J. -G. ;
Zhou, J. -S. ;
Goodenough, J. B. ;
Zhou, H. D. ;
Matsubayashi, K. ;
Uwatoko, Y. ;
Kong, P. P. ;
Jin, C. Q. ;
Yang, W. G. ;
Shen, G. Y. .
PHYSICAL REVIEW LETTERS, 2012, 108 (23)
[5]   A new method for measuring the degree of preferred orientation in bulk textured YBa2Cu3Ox [J].
Leventouri, T .
PHYSICA C, 1997, 277 (1-2) :82-86
[6]   Electronic structure and magnetism of La4Ni3O8 from first principles [J].
Liu, Ting ;
Zhang, Guoren ;
Zhang, Xiaoli ;
Jia, Ting ;
Zeng, Zhi ;
Lin, H. Q. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2012, 24 (40)
[7]   ABSENCE OF FERROMAGNETISM OR ANTIFERROMAGNETISM IN ONE- OR 2-DIMENSIONAL ISOTROPIC HEISENBERG MODELS [J].
MERMIN, ND ;
WAGNER, H .
PHYSICAL REVIEW LETTERS, 1966, 17 (22) :1133-&
[8]   NUCLEAR SPIN-LATTICE RELAXATION IN HEXAGONAL TRANSITION METALS - TITANIUM [J].
NARATH, A .
PHYSICAL REVIEW, 1967, 162 (02) :320-&
[9]   Pressure-induced metal-insulator and spin-state transition in low-valence layered nickelates [J].
Pardo, Victor ;
Pickett, Warren E. .
PHYSICAL REVIEW B, 2012, 85 (04)
[10]   Quantum Confinement Induced Molecular Correlated Insulating State in La4Ni3O8 [J].
Pardo, Victor ;
Pickett, Warren E. .
PHYSICAL REVIEW LETTERS, 2010, 105 (26)