Ammonia as a possible element in an energy infrastructure: catalysts for ammonia decomposition

被引：619

作者：

Schueth, F. ^{[1
]}

Palkovits, R. ^{[1
]}

Schloegl, R. ^{[2
]}

Su, D. S. ^{[2
]}

机构：

[1] MPI Kohlenforsch, D-45470 Mulheim, Germany

[2] Fritz Haber Inst MPG, D-14195 Berlin, Germany

来源：

ENERGY & ENVIRONMENTAL SCIENCE | 2012年 / 5卷 / 04期

关键词：

COX-FREE HYDROGEN; TUNGSTEN-BASED CATALYSTS; NH3; DECOMPOSITION; FUEL-CELL; BARIUM CERATE; RU CATALYSTS; EFFICIENT GENERATION; NI/SBA-15; CATALYST; STABLE CATALYSTS; CARBON NANOTUBES;

D O I：

10.1039/c2ee02865d

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The possible role of ammonia in a future energy infrastructure is discussed. The review is focused on the catalytic decomposition of ammonia as a key step. Other aspects, such as the catalytic removal of ammonia from gasification product gas or direct ammonia fuel cells, are highlighted as well. The more general question of the integration of ammonia in an infrastructure is also covered.

引用

页码：6278 / 6289

页数：12

共 133 条

[1] [Anonymous], 2006, AMMONIA ULLMANNS ENC
[2] [Anonymous], ULLMANNS ENCY IND CH
[3] [Anonymous], TARG ONB HYDR STOR S
[4] Micro-kinetic modeling of NH3 decomposition on Ni and its application to solid oxide fuel cells
Appari, Srinivas
Janardhanan, Vinod M.
Jayanti, Sreenivas
Maier, Lubow
Tischer, Steffen
Deutschmann, Olaf
[J]. CHEMICAL ENGINEERING SCIENCE, 2011, 66 (21) : 5184 - 5191
[5] Studies of the Kinetics of Two Parallel Reactions: Ammonia Decomposition and Nitriding of Iron Catalyst
Arabczyk, Walerian
Pelka, Rafat
[J]. JOURNAL OF PHYSICAL CHEMISTRY A, 2009, 113 (02) : 411 - 416
[6] High-temperature-stable catalysts by hollow sphere encapsulation
Arnal, Pablo M.
Comotti, Massimiliano
Schueth, Ferdi
[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2006, 45 (48) : 8224 - 8227
[7] Electrochemical promotion of Pd, Fe and distributed Pt catalyst-electrodes
Balomenou, S
Pitselis, G
Polydoros, D
Giannikos, A
Vradis, A
Frenzel, A
Pliangos, C
Pütter, H
Vayenas, CG
[J]. SOLID STATE IONICS, 2000, 136 : 857 - 862
[8] Why the optimal ammonia synthesis catalyst is not the optimal ammonia decomposition catalyst
Boisen, A
Dahl, S
Norskov, JK
Christensen, CH
[J]. JOURNAL OF CATALYSIS, 2005, 230 (02) : 309 - 312
[9] Kinetics of NH3 decomposition over well dispersed Ru
Bradford, MCJ
Fanning, PE
Vannice, MA
[J]. JOURNAL OF CATALYSIS, 1997, 172 (02) : 479 - 484
[10] Nanoengineering of inorganic and hybrid hollow spheres by colloidal templating
Caruso, F
Caruso, RA
Möhwald, H
[J]. SCIENCE, 1998, 282 (5391) : 1111 - 1114

← 1 2 3 4 5 6 7 8 9 10 →