Facile Synthesis of a Phosphorylcholine-Based Zwitterionic Amphiphilic Copolymer for Anti-Biofouling Coatings

被引：29

作者：

Seetho, Kellie ^{[1
,2
,3
]}

Zhang, Shiyi ^{[1
,2
,3
]}

Pollack, Kevin A. ^{[1
,2
,3
]}

Zou, Jiong ^{[1
,2
,3
]}

Raymond, Jeffery E. ^{[1
,2
,3
]}

Martinez, Edgar ^{[4
]}

Wooley, Karen L. ^{[1
,2
,3
]}

机构：

[1] Texas A&M Univ, Lab Synthet Biol Interact, Dept Chem, College Stn, TX 77842 USA

[2] Texas A&M Univ, Lab Synthet Biol Interact, Dept Chem Engn, College Stn, TX 77842 USA

[3] Texas A&M Univ, Lab Synthet Biol Interact, Dept Mat Sci & Engn, College Stn, TX 77842 USA

[4] Beclunan Coulter Particle Characterizat Lab, Miami, FL 33196 USA

来源：

ACS MACRO LETTERS | 2015年 / 4卷 / 05期

关键词：

PHOSPHOLIPID POLYMERS; PROTEIN ADSORPTION; SURFACE; MARINE; RESISTANCE; ROUGHNESS;

D O I：

10.1021/mz500818c

中图分类号：

O63 [高分子化学（高聚物）];

学科分类号：

070305 ; 080501 ; 081704 ;

摘要：

An antibiofouling polymer coating, combined with both zwitterionic and amphiphilic features, is engineered by a two-step modification of a commodity polymer. The surface properties of the resultant polymer coating can be easily tuned by varying the extent of cross-linking in the network. Higher antibiofouling efficiency was observed for these surfaces vs. an elastomeric polydimethylsiloxane standard (Sylgard 184) against the adsorption of biomacromolecules and a marine fouling organism (Ulva zoospores) has been demonstrated. This design establishes a platform for the achievement of functionalized amphiphilic zwitterionic copolymers from relatively inexpensive starting materials via simple chemical manipulations.

引用

页码：505 / 510

页数：6

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