Third-order nonlinear optical susceptibility measurement in 1-methyl-1′-octadecyl-2,2′-cyanine perchlorate Langmuir-Blodgett films by means of electroabsorption spectroscopy

被引:1
作者
Murakami, H
Morita, R
Watanabe, T
Asai, K
Honma, I
Zhou, HS
Yamashita, M
Ishigure, K
Shigekawa, H
机构
[1] Hokkaido Univ, Dept Appl Phys, Kita Ku, Sapporo, Hokkaido 0608628, Japan
[2] Univ Tokyo, Dept Quantum Engn & Syst Sci, Bunkyo Ku, Tokyo 1130032, Japan
[3] AIST, Electrotech Lab, Div Energy, Tsukuba, Ibaraki 3058568, Japan
[4] Univ Tsukuba, Inst Mat Sci, Ctr TARA, Tsukuba, Ibaraki 3058573, Japan
来源
MOLECULAR CRYSTALS AND LIQUID CRYSTALS SCIENCE AND TECHNOLOGY SECTION A-MOLECULAR CRYSTALS AND LIQUID CRYSTALS | 1999年 / 327卷
关键词
J-aggregate; Langmuir-Blodgett film; cyanine dye; electroabsorption spectroscopy; nonlinear optical susceptibility;
D O I
10.1080/10587259908026774
中图分类号
O7 [晶体学];
学科分类号
0702 ; 070205 ; 0703 ; 080501 ;
摘要
By an electroabsorption spectroscopy technique, we determined the third-order nonlinear optical susceptibilities dispersion in 1-methyl-1'-octadecyl-2,2'-cyanine perchlorate Langmuir-Blodgett (J-aggregate) films in the range of 1.8 to 2.7 eV. In addition, from the values of the polarizability change in the monomer and aggregate films, the number of molecules in an aggregate was evaluated to be 3-4.
引用
收藏
页码:31 / 35
页数:5
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