Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate

被引:320
作者
Shen, Yao [1 ,2 ]
Li, Yao-Dong [3 ]
Wo, Hongliang [1 ,2 ]
Li, Yuesheng [4 ]
Shen, Shoudong [1 ,2 ]
Pan, Bingying [1 ,2 ]
Wang, Qisi [1 ,2 ]
Walker, H. C. [5 ]
Steffens, P. [6 ]
Boehm, M. [6 ]
Hao, Yiqing [1 ,2 ]
Quintero-Castro, D. L. [7 ]
Harriger, L. W. [8 ]
Frontzek, M. D. [9 ]
Hao, Lijie [10 ]
Meng, Siqin [10 ]
Zhang, Qingming [4 ,11 ,12 ]
Chen, Gang [1 ,2 ,12 ,13 ]
Zhao, Jun [1 ,2 ,12 ]
机构
[1] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China
[2] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China
[3] Fudan Univ, Sch Comp Sci, Shanghai 200433, Peoples R China
[4] Renmin Univ China, Beijing Key Lab Optoelect Funct Mat & Micronano D, Dept Phys, Beijing 100872, Peoples R China
[5] STFC, Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England
[6] Inst Laue Langevin, 71 Ave Martyrs, F-38042 Grenoble 9, France
[7] Helmholtz Zentrum Berlin Mat & Energie, D-14109 Berlin, Germany
[8] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA
[9] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA
[10] China Inst Atom Energy, Neutron Scattering Lab, Beijing 102413, Peoples R China
[11] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai 200240, Peoples R China
[12] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
[13] Fudan Univ, Ctr Field Theory & Particle Phys, Shanghai 200433, Peoples R China
基金
中国国家自然科学基金;
关键词
VALENCE-BOND STATE; KAGOME-LATTICE; GROUND-STATE; EXCITATIONS; TOPOLOGY; PHYSICS;
D O I
10.1038/nature20614
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and quantum-information applications, and experimental identification of a quantum spin liquid state is of fundamental importance for our understanding of quantum matter. Theoretical studies have proposed various quantum-spin-liquid ground states1-4, most of which are characterized by exotic spin excitations with fractional quantum numbers (termed 'spinons'). Here we report neutron scattering measurements of the triangular-lattice antiferromagnet YbMgGaO4 that reveal broad spin excitations covering a wide region of the Brillouin zone. The observed diffusive spin excitation persists at the lowest measured energy and shows a clear upper excitation edge, consistent with the particle-hole excitation of a spinon Fermi surface. Our results therefore point to the existence of a quantum spin liquid state with a spinon Fermi surface in YbMgGaO4, which has a perfect spin-1/2 triangular lattice as in the original proposal(4) of quantum spin liquids.
引用
收藏
页码:559 / +
页数:13
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