Enhanced photocatalytic activity of Ag-TiO2/Ag heterogeneous films

被引:3
作者
Liang, Ying [1 ]
Wang, ShaoHua [1 ]
Guo, PengFeng [1 ]
机构
[1] Guangdong Pharmaceut Univ, Sch Chem & Chem Engn, Guangzhou 510006, Guangdong, Peoples R China
基金
中国国家自然科学基金;
关键词
heterogeneous films; Ag nanoparticles; Ag film; photocatalytic activity; ATOMIC LAYER DEPOSITION; TIO2; AG; NANOPARTICLES; PHOTODEGRADATION; NANOCOMPOSITES; PERFORMANCES;
D O I
10.1134/S0036024415110102
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Ag-deposited TiO2 and Ag (Ag-TiO2/Ag) films coated on glass substrates were prepared using a simple sol-gel and dip-coating method. The Ag chemical state was investigated through X-ray diffractometry and X-ray photoelectron spectroscopy. Results showed that the Ag mainly exists in metallic state in the Ag-TiO2 film. Ag-TiO2/Ag exhibits higher photocatalytic activity than individual Ag-TiO2 and TiO2/Ag films. This enhanced photocatalytic activity was attributed to high surface plasmon resonance effects and separation rates of photoinduced electron-hole pairs of Ag nanoparticles. Results were verified by photoluminescence and UV-Vis spectroscopy.
引用
收藏
页码:2137 / 2141
页数:5
相关论文
共 22 条
[1]   A New Route to Size and Population Control of Silver Clusters on Colloidal TiO2 Nanocrystals [J].
Cao-Thang Dinh ;
Thanh-Dinh Nguyen ;
Kleitz, Freddy ;
Trong-On Do .
ACS APPLIED MATERIALS & INTERFACES, 2011, 3 (07) :2228-2234
[2]   Ag-Nanoparticle-Decorated SiO2 Nanospheres Exhibiting Remarkable Plasmon-Mediated Photocatalytic Properties [J].
Chen, Kuang-Hsiu ;
Pu, Ying-Chih ;
Chang, Kao-Der ;
Liang, Yi-Fan ;
Liu, Chia-Ming ;
Yeh, Jien-Wei ;
Shih, Han-C. ;
Hsu, Yung-Jung .
JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (35) :19039-19045
[3]   Photocatalytic synthesis of silver nanoparticles stabilized by TiO2 nanorods:: A semiconductor/metal nanocomposite in homogeneous nonpolar solution [J].
Cozzoli, PD ;
Comparelli, R ;
Fanizza, E ;
Curri, ML ;
Agostiano, A ;
Laub, D .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2004, 126 (12) :3868-3879
[4]   Understanding the High Photocatalytic Activity of (B, Ag)-Codoped TiO2 under Solar-Light Irradiation with XPS, Solid-State NMR, and DFT Calculations [J].
Feng, Ningdong ;
Wang, Qiang ;
Zheng, Anmin ;
Zhang, Zhengfeng ;
Fan, Jie ;
Liu, Shang-Bin ;
Amoureux, Jean-Paul ;
Deng, Feng .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2013, 135 (04) :1607-1616
[5]   Photocatalysis of Ag-Loaded TiO2 Nanotube Arrays Formed by Atomic Layer Deposition [J].
Liang, Yu-Chuan ;
Wang, Chih-Chieh ;
Kei, Chi-Chung ;
Hsueh, Yang-Chih ;
Cho, Wen-Hao ;
Perng, Tsong-Pyng .
JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (19) :9498-9502
[6]   Hierarchical TiO2 Nanostructured Array/P3HT Hybrid Solar Cells with Interfacial Modification [J].
Liao, Wen-Pin ;
Hsu, Shu-Chien ;
Lin, Wan-Hsien ;
Wu, Jih-Jen .
JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (30) :15938-15945
[7]   Biomimetic Synthesis of TiO2-SiO2-Ag Nanocomposites with Enhanced Visible-Light Photocatalytic Activity [J].
Liu, Chuang ;
Yang, Dong ;
Jiao, Yang ;
Tian, Yao ;
Wang, Yuangui ;
Jiang, Zhongyi .
ACS APPLIED MATERIALS & INTERFACES, 2013, 5 (09) :3824-3832
[8]   UV-and Visible-Light Photocatalytic Activity of Simultaneously Deposited and Doped Ag/Ag(I)-TiO2 Photocatalyst [J].
Liu, Rui ;
Wang, Ping ;
Wang, Xuefei ;
Yu, Huogen ;
Yu, Jiaguo .
JOURNAL OF PHYSICAL CHEMISTRY C, 2012, 116 (33) :17721-17728
[9]   Fabrication and characteristics of visible light active TiO2 films by reduction treatment in carbon powder [J].
Lu, Y. ;
Hao, L. ;
Matsuzaka, K. ;
Pan, F. ;
Yoshida, H. .
MATERIALS TECHNOLOGY, 2013, 28 (04) :205-213
[10]   Effect of Metal Ions (Ag, Co, Ni, and Pd) on the Visible Light Degradation of Rhodamine B by Carbon-Covered Alumina-Supported TiO2 in Aqueous Solutions [J].
Mahlambi, Mphilisi M. ;
Mishra, Ajay K. ;
Mishra, Shivani B. ;
Krause, Rui W. ;
Mamba, Bhekie B. ;
Raichur, Ashok M. .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2013, 52 (05) :1783-1794