Removal and fate of micropollutants in a sponge-based moving bed bioreactor

被引:80
作者
Luo, Yunlong [1 ]
Guo, Wenshan [1 ]
Huu Hao Ngo [1 ]
Long Duc Nghiem [2 ]
Hai, Faisal Ibney [2 ]
Kang, Jinguo [2 ]
Xia, Siqing [3 ]
Zhang, Zhiqiang [3 ]
Price, William Evan [4 ]
机构
[1] Univ Technol Sydney, Sch Civil & Environm Engn, Ctr Technol Water & Wastewater, Sydney, NSW 2007, Australia
[2] Univ Wollongong, Sch Civil Min & Environm Engn, Strateg Water Infrastruct Lab, Wollongong, NSW 2522, Australia
[3] Tongji Univ, Coll Environm Sci & Engn, State Key Lab Pollut Control & Resource Reuse, Shanghai 200092, Peoples R China
[4] Univ Wollongong, AIIM, Strateg Water Infrastruct Lab, North Wollongong, NSW 2500, Australia
关键词
Micropollutants removal; Moving bed bioreactor (MBBR); Sponge; Attached-growth; Biodegradation; WASTE-WATER TREATMENT; PERSONAL CARE PRODUCTS; MEMBRANE BIOREACTOR; ACTIVATED CARBON; TREATMENT PLANTS; PHARMACEUTICALS; CONTAMINANTS; DEGRADATION; ESTROGENS; DRUGS;
D O I
10.1016/j.biortech.2014.02.107
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
This study investigated the removal of micropollutants using polyurethane sponge as attached-growth carrier. Batch experiments demonstrated that micropollutants could adsorb to non-acclimatized sponge cubes to varying extents. Acclimatized sponge showed significantly enhanced removal of some less hydrophobic compounds (logD < 2.5), such as ibuprofen, acetaminophen, naproxen, and estriol, as compared with non-acclimatized sponge. The results for bench-scale sponge-based moving bed bioreactor (MBBR) system elucidated compound-specific variation in removal, ranging from 25.9% (carbamazepine) to 96.8% (beta-Estradiol 17-acetate) on average. In the MBBR system, biodegradation served as a major removal pathway for most compounds. However, sorption to sludge phase was also a notable removal mechanism of some persistent micropollutants. Particularly, carbamazepine, ketoprofen and pentachlorophenol were found at high concentrations (7.87, 6.05 and 5.55 mu g/g, respectively) on suspended biosolids. As a whole, the effectiveness of MBBR for micropollutant removal was comparable with those of activated sludge processes and MBRs. (c) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:311 / 319
页数:9
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