Electrophoretic Deposition of Multi-walled Carbon Nanotube on a Stainless Steel Electrode for use in Sediment Microbial Fuel Cells

被引:16
作者
Song, Tian-shun [1 ]
Peng-Xiao [1 ]
Wu, Xia-yuan [1 ]
Zhou, Charles C. [1 ]
机构
[1] Nanjing Univ Technol, Coll Biotechnol & Pharmaceut Engn, Inst Joint Bioenergy, Nanjing 210009, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
Carbon nanotube; Sediment microbial fuel cell; Stainless steel; Electrophoretic deposition; FRESH-WATER SEDIMENT; ELECTRICITY-GENERATION; POWER; PERFORMANCE; COMMUNITIES; CATHODE; ENERGY; ANODE;
D O I
10.1007/s12010-013-0274-3
中图分类号
Q5 [生物化学]; Q7 [分子生物学];
学科分类号
071010 ; 081704 ;
摘要
Sediment microbial fuel cells (SMFCs) could be used as power sources and one type of new technology for the removal of organic matters in sediments. In order to improve electrode materials and enhance their effect on the performance, we deposited multi-walled carbon nanotube (MWNT) on stainless steel net (SSN). Electrophoretic deposition technique as a method with low cost, process simplicity, and thickness control was used for this electrode modification and produced this novel SSN-MWNT electrode. The performances of SMFCs with SSN-MWNT as electrode were investigated. The results showed that the maximum power density of SMFC with SSN-MWNT cathode was 31.6 mW m(-2), which was 3.2 times that of SMFC with an uncoated stainless steel cathode. However, no significant increase in the maximum power density of SMFC with SSN-MWNT anode was detected. Further electrochemical analysis showed that when SSN-MWNT was used as the cathode, the cathodic electrochemical activity and oxygen reduction rate were significantly improved. This study demonstrates that the electrophoretic deposition of carbon nanotubes on conductive substrate can be applied for improving the performance of SMFC.
引用
收藏
页码:1241 / 1250
页数:10
相关论文
共 31 条
[1]   Electrophoretic deposition of carbon nanotubes [J].
Boccaccini, Aldo R. ;
Cho, Johann ;
Roether, Judith A. ;
Thomas, Boris J. C. ;
Minay, E. Jane ;
Shaffer, Milo S. P. .
CARBON, 2006, 44 (15) :3149-3160
[2]   Electrode-reducing microorganisms that harvest energy from marine sediments [J].
Bond, DR ;
Holmes, DE ;
Tender, LM ;
Lovley, DR .
SCIENCE, 2002, 295 (5554) :483-485
[3]   HISTORY OF THE APPLICATION OF THE GENERALIZED LEWIS ACID-BASE THEORY TO METALS [J].
BREWER, L .
JOURNAL OF NUCLEAR MATERIALS, 1989, 167 :3-6
[4]   Characterisation of carbon nanotube films deposited by electrophoretic deposition [J].
Cho, Johann ;
Konopka, Katarzyna ;
Rozniatowski, Krzysztof ;
Garcia-Lecina, Eva ;
Shaffer, Milo S. P. ;
Boccaccini, Aldo R. .
CARBON, 2009, 47 (01) :58-67
[5]   Evaluation of biocathodes in freshwater and brackish sediment microbial fuel cells [J].
De Schamphelaire, Liesje ;
Boeckx, Pascal ;
Verstraete, Willy .
APPLIED MICROBIOLOGY AND BIOTECHNOLOGY, 2010, 87 (05) :1675-1687
[6]   Outlook for benefits of sediment microbial fuel cells with two bio-electrodes [J].
De Schamphelaire, Liesje ;
Rabaey, Korneel ;
Boeckx, Pascal ;
Boon, Nico ;
Verstraete, Willy .
MICROBIAL BIOTECHNOLOGY, 2008, 1 (06) :446-462
[7]   Batteryless, Wireless Sensor Powered by a Sediment Microbial Fuel Cell [J].
Donovan, Conrad ;
Dewan, Alim ;
Heo, Deukhyoun ;
Beyenal, Haluk .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008, 42 (22) :8591-8596
[8]   Marine microbial fuel cell:: Use of stainless steel electrodes as anode and cathode materials [J].
Dumas, C. ;
Mollica, A. ;
Feron, D. ;
Basseguy, R. ;
Etcheverry, L. ;
Bergel, A. .
ELECTROCHIMICA ACTA, 2007, 53 (02) :468-473
[9]   Checking graphite and stainless anodes with an experimental model of marine microbial fuel cell [J].
Dumas, Claire ;
Mollica, Alfonso ;
Feron, Damien ;
Basseguy, Regine ;
Etcheverry, Luc ;
Bergel, Alain .
BIORESOURCE TECHNOLOGY, 2008, 99 (18) :8887-8894
[10]   Bio-Electro-Fenton Process Driven by Microbial Fuel Cell for Wastewater Treatment [J].
Feng, Chun-Hua ;
Li, Fang-Bai ;
Mai, Hong-Jian ;
Li, Xiang-Zhong .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2010, 44 (05) :1875-1880