Hydrogen energy production from disposable chopsticks by a low temperature catalytic gasification

被引:21
作者
Chiang, Kung-Yuh [1 ]
Chien, Kuang-Li [1 ]
Lu, Cheng-Han [1 ]
机构
[1] Feng Chia Univ, Dept Environm Engn & Sci, Taichung 407, Taiwan
关键词
Gasification; Catalyst; Synthesis gas; Fluidized bed; FLUIDIZED-BED GASIFICATION; WOODY BIOMASS; AGGLOMERATION; REACTOR; COMBUSTION; CARBON; FUEL; GAS;
D O I
10.1016/j.ijhydene.2012.06.030
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
This study investigates the comparison of various mineral catalysts on the enhancement of energy yield efficiency with low temperature catalytic gasification of disposable chopsticks. The experiments were carried out in a fluidized bed reactor by controlling the temperature and keeping it within the range of 600 degrees C-800 degrees C. The mineral catalysts, such as aluminum silicate, zeolite and calcium oxide (CaO) were used as the experimental catalysts for enhancing energy yield in this research. According to the experimental results, the gasification temperature is a critical factor for improving the gas yield and quality. In general, a higher temperature provides more favorable conditions for thermal cracking and enhances the gas yield and quality. The hydrogen content produced from the tested biomass gasification by various catalysts slightly increased from 11.77% to 14.57%. Furthermore, the lower heating value of synthesis gas increased from 9.28 MJ/Nm(3) to 9.62 MJ/Nm(3), when the fluidized bed reactor temperature operated at 600 degrees C and the tested catalysts addition. That is, the catalytic gasification has good energy yield performance for enhancing higher energy content of synthesis gas in a lower-temperature catalytic fluidized bed reactor. Compared with the hydrogen production efficiency, the addition of a calcium based catalyst can reduce bed agglomeration tendency, but it also improves the energy yield in this research. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:15672 / 15680
页数:9
相关论文
共 32 条
  • [11] Biomass gasification with air in a fluidized bed:: Effect of the in-bed use of dolomite under different operation conditions
    Gil, J
    Caballero, MA
    Martín, JA
    Aznar, MP
    Corella, J
    [J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1999, 38 (11) : 4226 - 4235
  • [12] Gomez-Barea A., 2009, HDB COMBUSTION, V4
  • [13] Hydrogen production via CaO sorption enhanced anaerobic gasification of sawdust in a bubbling fluidized bed
    Han, Long
    Wang, Qinhui
    Yang, Yukun
    Yu, Chunjiang
    Fang, Mengxiang
    Luo, Zhongyang
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2011, 36 (08) : 4820 - 4829
  • [14] IEA, 2020, WORLD EN OUTL, V2050, DOI [DOI 10.1787/557A761B-EN, 10.1787/557a761b-en]
  • [15] Generation of hydrogen rich gas through fluidized bed gasification of biomass
    Karmakar, M. K.
    Datta, A. B.
    [J]. BIORESOURCE TECHNOLOGY, 2011, 102 (02) : 1907 - 1913
  • [16] Gasification of palm empty fruit bunch in a bubbling fluidized bed: A performance and agglomeration study
    Lahijani, Pooya
    Zainal, Zainal Alimuddin
    [J]. BIORESOURCE TECHNOLOGY, 2011, 102 (02) : 2068 - 2076
  • [17] Biomass gasification in a circulating fluidized bed
    Li, XT
    Grace, JR
    Lim, CJ
    Watkinson, AP
    Chen, HP
    Kim, JR
    [J]. BIOMASS & BIOENERGY, 2004, 26 (02) : 171 - 193
  • [18] The role of ash particles in the bed agglomeration during the fluidized bed combustion of rice straw
    Liu, Huanpeng
    Feng, Yujie
    Wu, Shaohua
    Liu, Dunyu
    [J]. BIORESOURCE TECHNOLOGY, 2009, 100 (24) : 6505 - 6513
  • [19] A sustainable woody biomass biorefinery
    Liu, Shijie
    Lu, Houfang
    Hu, Ruofei
    Shupe, Alan
    Lin, Lu
    Liang, Bin
    [J]. BIOTECHNOLOGY ADVANCES, 2012, 30 (04) : 785 - 810
  • [20] Bio-syngas production from biomass catalytic gasification
    Lv, Pengmei
    Yuan, Zhenhong
    Wu, Chuangzhi
    Ma, Longlong
    Chen, Yong
    Tsubaki, Noritatsu
    [J]. ENERGY CONVERSION AND MANAGEMENT, 2007, 48 (04) : 1132 - 1139