Recent Progress of Single-Atom Catalysts in the Electrocatalytic Reduction of Oxygen to Hydrogen Peroxide

被引：34

作者：

Zhu, Weiya ^{[1
,2
]}

Chen, Shaowei ^{[2
]}

机构：

[1] South China Univ Technol, Sch Mat Sci & Engn, Guangzhou 510031, Guangdong, Peoples R China

[2] Univ Calif Santa Cruz, Dept Chem & Biochem, 1156 High St, Santa Cruz, CA 95064 USA

来源：

ELECTROANALYSIS | 2020年 / 32卷 / 12期

基金：

美国国家科学基金会;

关键词：

single-atom catalyst; oxygen reduction reaction; hydrogen peroxide; selectivity; DIRECT H2O2 PRODUCTION; ACTIVE-SITES; DOPED CARBON; RATIONAL DESIGN; O-2; REDUCTION; 2-ELECTRON; GRAPHENE; EFFICIENCY; WATER; FE;

D O I：

10.1002/elan.202060334

中图分类号：

O65 [分析化学];

学科分类号：

070302 ; 081704 ;

摘要：

Single-atom catalysts (SACs) have been attracting extensive interest in the electrocatalytic production of hydrogen peroxide by oxygen reduction reaction (ORR). This is due to the maximal efficiency of atom utilization and intimate interaction of the metal centers with the supporting matrix that may be exploited for deliberate manipulation of the electrocatalytic activity and selectivity, in comparison with the conventional nanoparticle counterparts. Herein, we summarize recent progress of the design and engineering of SACs towards ORR for H(2)O(2)generation, based on both noble and non-noble metals. We conclude the review with a perspective highlighting the promises and challenges involved in future research.

引用

页码：2591 / 2602

页数：12

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