Coupling of spin and lattice modes in the S=1/2 two-dimensional antiferromagnet K2V3O8 with magneto-dielectric couplings

被引:12
作者
Choi, K. -Y. [1 ]
Lemmens, P. [2 ]
Gnezdilov, V. P. [3 ]
Sales, B. C. [4 ]
Lumsden, M. D. [4 ]
机构
[1] Chung Ang Univ, Dept Phys, Seoul 156756, South Korea
[2] Tech Univ Carolo Wilhelmina Braunschweig, Inst Condensed Matter Phys, D-38106 Braunschweig, Germany
[3] BI Verkin Inst Low Temp Phys NASU, UA-61164 Kharkov, Ukraine
[4] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA
关键词
CRYSTAL-STRUCTURE; POLARIZATION; TEMPERATURE; SPECTRA;
D O I
10.1103/PhysRevB.85.144434
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Lattice dynamics and magnetic excitations are investigated to elucidate the origin of magneto-dielectric effects in the S = 1/2 two-dimensional quantum spin compound K2V3O8. We find evidence for lattice instabilities at 110 K and 60 K as optical phonon anomalies and a soft mode at 26 cm(-1) in A(1) symmetry. Two-magnon excitations in B-1 symmetry show an unconventional double-peak structure and temperature dependence. This suggests the existence of a split mode near the zone boundary caused by a mixing of spin and lattice modes.
引用
收藏
页数:6
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