共 32 条
Investigations of lithium-sulfur batteries using electrochemical impedance spectroscopy
被引:364
作者:

Canas, Natalia A.
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German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany
Univ Stuttgart, Inst Thermodynam & Thermal Engn, Stuttgart, Germany German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany

Hirose, Kei
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German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany

Pascucci, Brigitta
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German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany
Univ Appl Sci Esslingen, Fac Basic Sci, Esslingen, Germany German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany

Wagner, Norbert
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German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany

Friedrich, K. Andreas
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German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany
Univ Stuttgart, Inst Thermodynam & Thermal Engn, Stuttgart, Germany German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany

Hiesgen, Renate
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Univ Appl Sci Esslingen, Fac Basic Sci, Esslingen, Germany German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany
机构:
[1] German Aerosp Ctr, Inst Tech Thermodynam, Stuttgart, Germany
[2] Univ Stuttgart, Inst Thermodynam & Thermal Engn, Stuttgart, Germany
[3] Univ Appl Sci Esslingen, Fac Basic Sci, Esslingen, Germany
关键词:
Lithium-sulfur battery;
Electrochemical impedance spectroscopy;
Degradation;
CATHODE;
ELECTRODE;
PERFORMANCE;
COMPOSITE;
CELL;
D O I:
10.1016/j.electacta.2013.02.101
中图分类号:
O646 [电化学、电解、磁化学];
学科分类号:
081704 ;
摘要:
The electrochemical behavior of lithium-sulfur (Li-S) batteries was investigated by means of electrochemical impedance spectroscopy (EIS). Measurements were performed in equidistant charge intervals at different depths of discharge and charge during the first cycle. Additionally, the degradation of the cells was analyzed for up to 50 cycles. An equivalent electrical circuit is proposed to simulate the electrochemical processes and to quantify the impedance contributions of Li-S batteries. EIS as a function of the cycle number shows an increased capacity for fading correlated with a decrease in the charge transfer resistance of the cathode. Atomic force microscopy (AFM) was also used to provide information about changes in the electrical conductivity of the cathode surface as they are related to the building of isolating films.(C) 2013 Elsevier Ltd. All rights reserved.
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页码:42 / 51
页数:10
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