Morphological transitions of active Brownian particle aggregates on porous walls

被引:15
作者
Das, Suchismita [1 ]
Chelakkot, Raghunath [1 ]
机构
[1] Indian Inst Technol, Dept Phys, Mumbai, Maharashtra, India
关键词
PRESSURE; DYNAMICS; MOTION; DEFECTS;
D O I
10.1039/d0sm00797h
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Motility-induced wall aggregation of Active Brownian Particles (ABPs) is a well-studied phenomenon. Here, we study the aggregation of ABPs on porous walls, which allows the particles to penetrate through at large motility. We show that the active aggregates undergo a morphological transition from a connected dense-phase to disconnected droplets with an increase in wall porosity and the particle self-motility, similar to wetting-dewetting transitions in equilibrium fluids. We show that both morphologically distinct states are stable, and independent of initial conditions at least in some parameter regions. Our analysis reveals that changes in wall porosity affect the intrinsic properties of the aggregates and changes the effective wall-aggregate interfacial tension, consistent with the appearance of the morphological transition. Accordingly, a close analysis of the density, as well as orientational distribution, indicates that the underlying reason for such morphological transitions is not necessarily specific to the systems with porous walls, and it can be possible to observe in a larger class of confined, active systems by tuning the properties of confining walls.
引用
收藏
页码:7250 / 7255
页数:6
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