Growth rates of fine aerosol particles at a site near Beijing in June 2013

被引:49
作者
Zhao, Chuanfeng [1 ,2 ,3 ]
Li, Yanan [1 ,2 ]
Zhang, Fang [1 ,2 ]
Sun, Yele [4 ]
Wang, Pucai [4 ]
机构
[1] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China
[2] Beijing Normal Univ, Coll Global Change & Earth Syst Sci, Beijing 100875, Peoples R China
[3] Joint Ctr Global Change Studies, Beijing 100875, Peoples R China
[4] Chinese Acad Sci, Inst Atmospher Phys, Beijing 100875, Peoples R China
基金
中国国家自然科学基金;
关键词
growth rate; fine aerosol particle; Xianghe; SIZE DISTRIBUTIONS; LONG-TERM; SULFURIC-ACID; NUMBER-SIZE; NUCLEATION; CHINA; POLLUTION; EVENTS; H2SO4;
D O I
10.1007/s00376-017-7069-3
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Growth of fine aerosol particles is investigated during the Aerosol-CCN-Cloud Closure Experiment campaign in June 2013 at an urban site near Beijing. Analyses show a high frequency (similar to 50%) of fine aerosol particle growth events, and show that the growth rates range from 2.1 to 6.5 nm h-1 with a mean value of similar to 5.1 nm h(-1). A review of previous studies indicates that at least four mechanisms can affect the growth of fine aerosol particles: vapor condensation, intramodal coagulation, extramodal coagulation, and multi-phase chemical reaction. At the initial stage of fine aerosol particle growth, condensational growth usually plays a major role and coagulation efficiency generally increases with particle sizes. An overview of previous studies shows higher growth rates over megacity, urban and boreal forest regions than over rural and oceanic regions. This is most likely due to the higher condensational vapor, which can cause strong condensational growth of fine aerosol particles. Associated with these multiple factors of influence, there are large uncertainties for the aerosol particle growth rates, even at the same location.
引用
收藏
页码:209 / 217
页数:9
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