Surface chemistry of CO2 - Adsorption of carbon dioxide on clean surfaces at ultrahigh vacuum

被引:159
作者
Burghaus, Uwe [1 ]
机构
[1] NDSU Dept 2735, Dept Chem & Biochem, Fargo, ND 58108 USA
关键词
CO2; Surfaces; Carbonates; Gas-surface interactions; Heterogeneous catalysis; Greenhouse gas; MOLECULAR-BEAM SCATTERING; DENSITY-FUNCTIONAL THEORY; MONTE-CARLO SIMULATIONS; THERMAL-DESORPTION SPECTROSCOPY; VIBRATIONAL-SPECTRA; ADSORBED OXYGEN; OXIDE SURFACES; ELECTRON-BEAM; METHANOL ADSORPTION; MODEL CATALYSTS;
D O I
10.1016/j.progsurf.2014.03.002
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Carbon dioxide chemistry has attracted significant interest in recent years. Although the field is diverse, a current and more comprehensive review of the surface science literature may be of interest for a variety of communities since environmental chemistry, energy technology, materials science, catalysis, and nanocatalysis are certainly affected by gas-surface properties. The review describes surface phenomena and characterization strategies highlighting similarities and differences, instead of providing only a list of system-specific information. The various systems are roughly distinguished as those that clearly form carbonates and those that merely physisorb CO2 at ultra-high vacuum conditions. Nevertheless, extended sections about specific systems including rarely studied surfaces and unusual materials are included, making this review also useful as a reference. (C) 2014 Elsevier Ltd. All rights reserved.
引用
收藏
页码:161 / 217
页数:57
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