Polytetrafluoroethylene modifying: A low cost and easy way to improve the H2O resistance ability over MnOx for low-temperature NH3-SCR

被引:39
作者
Zhang, Ningqiang [1 ]
Li, Lingcong [1 ]
Zhang, Bingbing [3 ]
Sun, Yanming [1 ]
Song, Liyun [1 ]
Wu, Rui [1 ]
He, Hong [1 ,2 ]
机构
[1] Beijing Univ Technol, Beijing Key Lab Green Catalysis & Separat, Key Lab Beijing Reg Air Pollut Control, Beijing 100124, Peoples R China
[2] Collaborat Innovat Ctr Elect Vehicles Beijing, Beijing 100081, Peoples R China
[3] Inner Mongolia Univ, Sch Chem & Chem Engn, Hohhot 010021, Peoples R China
来源
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING | 2019年 / 7卷 / 03期
关键词
SCR; MnOx; Polytetrafluoroethylene; H2O resistance; Hydrophobic surface; SELECTIVE CATALYTIC-REDUCTION; NO; NH3; MECHANISM; SO2;
D O I
10.1016/j.jece.2019.103044
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Herein, an easy and low cost way is proposed to improve the H2O resistance ability of MnOx catalyst for low-temperature selective catalytic reduction (SCR), via PTFE modifying. The introduction of PTFE to MnOx promoted more tightly packed nanowires, generating a more hydrophobic surface. Mn-PTFE catalysts displayed H2O and SO2 resistance, lowering the probability of surface active sites being consumed. This work provides a new insight into the design of novel Mn-based composite catalysts with H2O and SO2 resistance ability, as well as promoting practical applications of Mn-based catalysts in low temperature SCR.
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页数:3
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