Feasibility of in-plane GDL structuration: Impact on current density distribution in large-area Proton Exchange Membrane Fuel Cells

被引:19
作者
Jabbour, Lara [1 ]
Robin, Christophe [1 ,2 ,3 ,4 ]
Nandjou, Fredy [1 ,2 ,3 ]
Vincent, Remi [1 ]
Micoud, Fabrice [1 ]
Poirot-Crouvezier, Jean-Philippe [1 ]
d'Arbigny, Julien [4 ]
Gerard, Mathias [1 ]
机构
[1] Univ Grenoble Alpes, CEA, LITEN, F-38054 Grenoble, France
[2] Univ Grenoble Alpes, LEPMI, F-38000 Grenoble, France
[3] CNRS, LEPMI, F-38000 Grenoble, France
[4] Zodiac Aerosp, F-78370 Plaisir, France
关键词
PEMFCs; Current density distribution; GDL structuration; Performance heterogeneities; Printed circuit board; GAS-DIFFUSION LAYER; WATER MANAGEMENT; CATALYST LAYERS; CATHODE; PEMFC; TEMPERATURE; GRADIENTS; ISSUES; MODEL;
D O I
10.1016/j.jpowsour.2015.09.043
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In the present work, the in-plane structuration of the electrode Gas Diffusion Layer (GDL) is proposed as an interesting approach to reduce the operating heterogeneities occurring within the cell along the gas flow fields, especially in dry operating conditions. This is especially important for transportation applications where the fuel cell is often operated in these conditions. Structured and homogeneous large-area (220 cm(2)) membrane electrode assemblies (MEAs) are tested in single-cell and 6-cell stack configurations. An S++(R) electronic card inserted in the stack is used to measure the current distribution within the cell, which is an indicator of the local electrochemical reaction conditions. The results of the current distribution measurements together with the cell performances obtained for the structured and the homogenous MEAs indicate that the electrode in-plane structuration is effective in reducing the functioning heterogeneities within the cell under specific operating conditions. (C) 2015 Elsevier B.V. All rights reserved.
引用
收藏
页码:380 / 390
页数:11
相关论文
共 32 条
[1]   Measurement of current distribution in a proton exchange membrane fuel cell with various flow arrangements - A parametric study [J].
Alaefour, Ibrahim ;
Karimi, G. ;
Jiao, Kui ;
Li, X. .
APPLIED ENERGY, 2012, 93 :80-89
[2]  
Asman C. P., Patent, Patent No. [WO 1997008766 A3, 1997008766]
[3]   On the role of fuel cells and hydrogen in a more sustainable and renewable energy future [J].
Brouwer, Jacob .
CURRENT APPLIED PHYSICS, 2010, 10 :S9-S17
[4]   A numerical analysis of PEMFC stack assembly through a 3D finite element model [J].
Carral, Christophe ;
Mele, Patrice .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2014, 39 (09) :4516-4530
[5]   Novel gas diffusion layer with water management function for PEMFC [J].
Chen, J ;
Matsuura, T ;
Hori, M .
JOURNAL OF POWER SOURCES, 2004, 131 (1-2) :155-161
[6]   Numerical modeling and experimental study of the influence of GDL properties on performance in a PEMFC [J].
Chun, Jeong Hwan ;
Park, Ki Tae ;
Jo, Dong Hyun ;
Kim, Sang Gon ;
Kim, Sung Hyun .
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2011, 36 (02) :1837-1845
[7]   Gas diffusion layer for proton exchange membrane fuel cells-A review [J].
Cindrella, L. ;
Kannan, A. M. ;
Lin, J. F. ;
Saminathan, K. ;
Ho, Y. ;
Lin, C. W. ;
Wertz, J. .
JOURNAL OF POWER SOURCES, 2009, 194 (01) :146-160
[8]   Durability and degradation issues of PEM fuel cell components [J].
de Bruijn, F. A. ;
Dam, V. A. T. ;
Janssen, G. J. M. .
FUEL CELLS, 2008, 8 (01) :3-22
[10]   Effects of Cathode Corrosion on Through-Plane Water Transport in Proton Exchange Membrane Fuel Cells [J].
Fairweather, Joseph D. ;
Spernjak, Dusan ;
Weber, Adam Z. ;
Harvey, David ;
Wessel, Silvia ;
Hussey, Daniel S. ;
Jacobson, David L. ;
Artyushkova, Kateryna ;
Mukundan, Rangachary ;
Borup, Rodney L. .
JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2013, 160 (09) :F980-F993