Synthesis of novel Ag/Ag2O heterostructures with solar full spectrum (UV, visible and near-infrared) light-driven photocatalytic activity and enhanced photoelectrochemical performance
被引:67
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作者:
Yang, Hongru
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机构:
Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R ChinaShandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China
Yang, Hongru
[1
]
Tian, Jian
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Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R ChinaShandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China
Tian, Jian
[1
]
Li, Tong
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Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R ChinaShandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China
Li, Tong
[1
]
Cui, Hongzhi
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Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R ChinaShandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China
Cui, Hongzhi
[1
]
机构:
[1] Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China
Solar full spectrum;
Ag2O;
Photocatalytic;
Mott-Schottky heterojunction;
Photoelectrochemical performance;
MOTT-SCHOTTKY HETEROJUNCTIONS;
RESPONSIVE ACTIVITY;
HYDROGEN EVOLUTION;
COUNTER ELECTRODES;
N HETEROJUNCTION;
TIO2;
NANOBELTS;
NANOPARTICLES;
DEGRADATION;
STABILITY;
MECHANISM;
D O I:
10.1016/j.catcom.2016.09.013
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Here we report the facile synthesis of Ag/Ag2O heterostructures, which exhibit excellent solar full spectrum (UV, visible and near-infrared) photocatalytic activity and an enhanced photoelectrochemical (PEC) performance under irradiation of near-infrared light. The improved photocatalytic property and PEC performance originated from the synergistic effect on the narrow band gap of Ag2O, plasmon enhancement of metallic Ag in-situ reduced from Ag2O, and metal-semiconductor (Ag-Ag2O) Mott-Schottky heterojunction. (C) 2016 Elsevier B.V. All rights reserved.
机构:
Kongju Natl Univ, Dept Adv Mat Engn, Cheonan 31080, South Korea
Kongju Natl Univ, Smart Nat Space Res Ctr, Cheonan 31080, South KoreaKongju Natl Univ, Dept Adv Mat Engn, Cheonan 31080, South Korea
机构:
Fujian Normal Univ, Dept Chem, Fuzhou 350007, Peoples R ChinaFujian Normal Univ, Dept Chem, Fuzhou 350007, Peoples R China
Cui, Duo Heng
Zheng, Yi Fan
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机构:
Zhejiang Univ Technol, Res Ctr Anal & Measurement, Hangzhou 310014, Zhejiang, Peoples R ChinaFujian Normal Univ, Dept Chem, Fuzhou 350007, Peoples R China
Zheng, Yi Fan
Song, Xu Chun
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机构:
Fujian Normal Univ, Dept Chem, Fuzhou 350007, Peoples R ChinaFujian Normal Univ, Dept Chem, Fuzhou 350007, Peoples R China