Thermophoretically induced flow field around a colloidal particle

被引:57
作者
Yang, Mingcheng [1 ]
Ripoll, Marisol [1 ]
机构
[1] Forschungszentrum Julich, Inst Complex Syst, D-52425 Julich, Germany
关键词
MULTIPARTICLE COLLISION DYNAMICS; THERMAL-DIFFUSION; MOLECULAR-DYNAMICS; CHARGED COLLOIDS; SIMULATION; MICROFLUIDICS; TRANSPORT; SYSTEMS; CHAIN; MODEL;
D O I
10.1039/c3sm27949a
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A colloidal particle suspended in a fluid solvent with a non-homogeneous temperature undergoes a thermophoretic force. This force may translate into a directed drift of the particle and a source-dipole-like flow field around it. Alternatively, if the colloid is fixed in space, the accompanying flow is long-ranged. In this work, we provide a first simulation study of the thermophoretic force-induced flow fields by a particle-based mesoscopic method. The simulation results are quantitatively consistent with theoretical predictions obtained by solving hydrodynamic equations. Based on these results, we propose a single-particle microfluidic pump without movable parts, in which the flow direction can be reversed. Furthermore, we quantify the long-range hydrodynamic attraction between two suspended particles near the boundary wall induced by the thermophoretic flow field.
引用
收藏
页码:4661 / 4671
页数:11
相关论文
共 70 条