Nucleation, growth and transport modelling of helium bubbles under nuclear irradiation in lead-lithium with the self-consistent nucleation theory and surface tension corrections

被引:5
作者
Fradera, J. [1 ]
Cuesta-Lopez, S. [1 ]
机构
[1] Univ Burgos UBU, Burgos 09001, Spain
关键词
Nuclear fusion; Liquid metals; CFD modelling; Helium cavitation; Nucleation; Surface tension; HOMOGENEOUS NUCLEATION; FREE-ENERGY; CURVATURE; GAS;
D O I
10.1016/j.fusengdes.2013.08.005
中图分类号
TL [原子能技术]; O571 [原子核物理学];
学科分类号
0827 ; 082701 ;
摘要
Helium (He) nucleation in liquid metal breeding blankets of a DT fusion reactor may have a significant impact regarding system design, safety and operation. Large He production rates are expected due to tritium (T) fuel self-sufficiency requirement, as both, He and T, are produced at the same rate. Low He solubility, local high concentrations, radiation damage and fluid discontinuities, among other phenomena, may yield the necessary conditions for He nucleation. Hence, He nucleation may have a significant impact on T inventory and may lower the T breeding ratio. A model based on the self-consistent nucleation theory (SCT) with a surface tension curvature correction model has been implemented in OpenFOAM (R) CFD code. A modification through a single parameter of the necessary nucleation condition is proposed in order to take into account all the nucleation triggering phenomena, specially radiation induced nucleation. Moreover, the kinetic growth model has been adapted so as to allow for the transition from a critical cluster to a macroscopic bubble with a diffusion growth process. Limitations and capabilities of the models are shown by means of zero-dimensional simulations and sensitivity analyses to key parameters under HCLL breeding unit conditions. Results provide a good qualitative insight into the helium nucleation phenomenon in LM systems for fusion technology and reinforces the idea that nucleation may not be a remote phenomenon, may have a large impact on the system's design and reveals the necessity to conduct experiments on He cavitation. (C) 2013 Published by Elsevier B.V.
引用
收藏
页码:3215 / 3223
页数:9
相关论文
共 32 条
[1]  
[Anonymous], 1975, KINETIC THEORY LIQUI
[2]   Tolman's δ, surface curvature, compressibility effects, and the free energy of drops [J].
Bartell, LS .
JOURNAL OF PHYSICAL CHEMISTRY B, 2001, 105 (47) :11615-11618
[3]   Numeric implementation of a nucleation, growth and transport model for helium bubbles in lead-lithium HCLL breeding blanket channels: Theory and code development [J].
Batet, L. ;
Fradera, J. ;
Mas de les Valls, E. ;
Sedano, L. A. .
FUSION ENGINEERING AND DESIGN, 2011, 86 (4-5) :421-428
[4]   Cavitation in liquid metals under negative pressures. Molecular dynamics modeling and simulation [J].
Bazhirov, T. T. ;
Norman, G. E. ;
Stegailov, V. V. .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2008, 20 (11)
[5]   Thermodynamic expressions for the Tolman length [J].
Blokhuis, EM ;
Kuipers, J .
JOURNAL OF CHEMICAL PHYSICS, 2006, 124 (07)
[6]  
Conrad R., 1988, FUSION TECHNOL, P1046
[7]  
Donnelly S. E., 1985, Radiation Effects, V90, P1, DOI 10.1080/00337578508222514
[8]   ON THE STABILITY OF GAS BUBBLES IN LIQUID-GAS SOLUTIONS [J].
EPSTEIN, PS ;
PLESSET, MS .
JOURNAL OF CHEMICAL PHYSICS, 1950, 18 (11) :1505-1509
[9]   Atomistic molecular point of view for liquid lead and lithium in Nuclear Fusion technology [J].
Fraile, A. ;
Cuesta-Lopez, S. ;
Iglesias, R. ;
Caro, A. ;
Perlado, J. M. .
JOURNAL OF NUCLEAR MATERIALS, 2013, 440 (1-3) :98-103
[10]   SELF-CONSISTENCY CORRECTION TO HOMOGENEOUS NUCLEATION THEORY - COMMENT [J].
GIRSHICK, SL .
JOURNAL OF CHEMICAL PHYSICS, 1991, 94 (01) :826-827