Polycyclic aromatic hydrocarbons (PAHs) in atmospheric dustfall from the industrial corridor in Hubei Province, Central China

被引:49
|
作者
Zhang, Jiaquan [1 ,2 ]
Qu, Chengkai [3 ,4 ]
Qi, Shihua [3 ]
Cao, Junji [2 ]
Zhan, Changlin [1 ,2 ]
Xing, Xinli [3 ]
Xiao, Yulun [1 ]
Zheng, Jingru [1 ]
Xiao, Wensheng [1 ]
机构
[1] Hubei Polytech Univ, Sch Environm Sci & Engn, Hubei Key Lab Mine Environm Pollut Control & Reme, Huangshi 435003, Peoples R China
[2] Chinese Acad Sci, Inst Earth Environm, Key Lab Aerosol Chem & Phys, Xian 710075, Peoples R China
[3] China Univ Geosci, State Key Lab Biogeol & Environm Geol, Wuhan 430074, Peoples R China
[4] Univ Naples Federico II, Dipartimento Scienze Terra Ambiente & Risorse, I-80134 Naples, Italy
关键词
Polycyclic aromatic hydrocarbons (PAHs); Dustfall; Industrial corridor; Source apportionment; Health risk assessment; RIVER-DELTA REGION; SOURCE APPORTIONMENT; RISK-ASSESSMENT; AGRICULTURAL SOILS; EMISSION FACTORS; SHANGHAI; IDENTIFICATION; ENVIRONMENT; PLAIN; AIR;
D O I
10.1007/s10653-014-9647-y
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Thirty atmospheric dustfall samples collected from an industrial corridor in Hubei Province, central China, were analyzed for 16 USEPA priority polycyclic aromatic hydrocarbons (PAHs) to investigate their concentrations, spatial distributions, sources, and health risks. Total PAH concentrations (I PAHs) pound ranged from 1.72 to 13.17 A mu g/g and averaged 4.91 A mu g/g. High molecular weight (4-5 rings) PAHs averaged 59.67 % of the I PAHs pound. Individual PAH concentrations were not significantly correlated with total organic carbon, possibly due to the semi-continuous inputs from anthropogenic sources. Source identification studies suggest that the PAHs were mainly from motor vehicles and biomass/coal combustion. The incremental lifetime cancer risks associated with exposure to PAHs in the dustfall ranged from 10(-4) to 10(-6); these indicate potentially serious carcinogenic risks for exposed populations in the industrial corridor.
引用
收藏
页码:891 / 903
页数:13
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