Synergistic effect of manganese dioxide and diatomite for fast decolorization and high removal capacity of methyl orange

被引:41
作者
Peng, Hui Hua [1 ]
Chen, Jie [1 ]
Jiang, De Yi [1 ]
Li, Min [2 ]
Feng, Li [3 ]
Losic, Dusan [4 ]
Dong, Fan [5 ]
Zhang, Yu Xin [1 ,3 ]
机构
[1] Chongqing Univ, Coll Resources & Environm Sci, State Key Lab Coal Mine Disaster Dynam & Control, Chongqing 400044, Peoples R China
[2] Chongqing Univ, Coll Optoelect Engn, Key Lab Fundamental Sci Micro Nanodevices & Syst, Chongqing 400044, Peoples R China
[3] Chongqing Univ, Coll Mat Sci & Engn, Key Lab Fundamental Sci Micro Nanodevices & Syst, Chongqing 400044, Peoples R China
[4] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia
[5] Chongqing Technol & Business Univ, Coll Environm & Resources, Chongqing Key Lab Catalysis & Funct Organ Mol, Chongqing 400067, Peoples R China
基金
高等学校博士学科点专项科研基金; 中国国家自然科学基金;
关键词
Manganese dioxide; Diatomite; Methyl orange; Decolorization; Wastewater treatment; LAYERED DOUBLE HYDROXIDES; PH-DEPENDENT DEGRADATION; AQUEOUS-SOLUTION; DIATOMACEOUS-EARTH; BASIC DYE; ADSORPTION; PERFORMANCE; SORPTION; WATER; OXIDE;
D O I
10.1016/j.jcis.2016.08.057
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
MnO2 nanostructures with two different morphologies (nanowires and nanosheets) were uniformly deposited on diatomite via a one-pot hydrothermal method. The fast decolorization and high removal capacity for anionic dye-MO over synthesized composites had been clarified. The results revealed that the equilibrium time was shortened to as low as 10-30 min, and the maximum adsorption capacities were 325 mg g(-1) and 420 mg g(-1) for nanowires and nanosheets composites, respectively, under the condition of initial pH 3 and ambient temperature. Indeed, the proposed decolorization mechanism was considered to be simultaneous multi-processes during the dye removal, including physical, physicochemical and chemical process. In principle, well-controlled cost-effective composites have promising ability to remove anionic dye pollutants for environmental remediation. (C) 2016 Elsevier Inc. All rights reserved.
引用
收藏
页码:1 / 9
页数:9
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