Occurrence and behavior of natural and anthropogenic (emerging and historical) halogenated compounds in marine biota from the Coast of Concepcion (Chile)

被引：33
作者：
Baron, Enrique [1 ]
Rudolph, Ignacio [2 ]
Chiang, Gustavo [2 ]
Barra, Ricardo [2 ]
Eljarrat, Ethel [1 ]
Barcelo, Damia [1 ,3 ]
机构：
[1] IDAEA CSIC, Dep Environm Chem, Water & Soil Qual Res Grp, Barcelona 08034, Spain
[2] Univ Concepcion, EULA Chile Environm Sci Ctr, Concepcion, Chile
[3] Univ Girona, Catalan Inst Water Res ICRA, Girona 17003, Spain
来源：
SCIENCE OF THE TOTAL ENVIRONMENT | 2013年 / 461卷
关键词：
Polybrominated diphenyl ethers (PBDEs); Methoxylated PBDEs; Halogenated norbornenes; Marine food web; Bioaccumulation; Biomagnification; POLYBROMINATED DIPHENYL ETHERS; ISOMER-SPECIFIC BIOACCUMULATION; PRESSURIZED LIQUID EXTRACTION; DECHLORANE PLUS; FLAME RETARDANTS; BLUE MUSSELS; TROPHIC TRANSFER; LLOBREGAT RIVER; PBDES; METABOLITES;
D O I：
10.1016/j.scitotenv.2013.05.006
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
Fifty-five biota samples from the Coast of Concepcion (Chile) were analyzed for PBDEs, emerging brominated FRs, halogenated norbornenes and naturally-occurring MeO-PBDEs. PBDEs, MeO-PBDEs and halogenated norbornenes were detected at concentration levels ranging from 11 to 170, nd to 118 and nd to 5.8 ng/g lw, respectively. However, emerging brominated FRs such as decabromodiphenylethane (DBDPE), hexabromobenzene (HBB) and pentabromoethylbenzene (PBEB) were not detected in any sample. Bioaccumulation and bioconcentration processes were evaluated for the different families of compounds. Biomagnification factors (BMFs) were calculated, and some PBDE congeners (BDE-28, BDE-183 and BDE-209) as well as MeO-PBDEs presented BMF > 1, being values of the naturally occurring MeO-PBDEs higher than those obtained for PBDEs. As regards halogenated norbornenes, BMF < 1 were found. (C) 2013 Elsevier B.V. All rights reserved.
引用
收藏
页码：258 / 264
页数：7
相关论文
共 58 条
[1]   Natural and anthropogenically-produced brominated compounds in endemic dolphins from Western South Atlantic: Another risk to a vulnerable species [J].
Alonso, Mariana B. ;
Eljarrat, Ethel ;
Gorga, Marina ;
Secchi, Eduardo R. ;
Bassoi, Manuela ;
Barbosa, Lupercio ;
Bertozzi, Carolina P. ;
Marigo, Juliana ;
Cremer, Marta ;
Domit, Camila ;
Azevedo, Alexandre F. ;
Dorneles, Paulo R. ;
Torres, Joao Paulo M. ;
Lailson-Brito, Jose ;
Malm, Olaf ;
Barcelo, Damia .
ENVIRONMENTAL POLLUTION, 2012, 170 :152-160
[2]   Polybrominated diphenyl ethers (PBDEs) and bioaccumulative hydroxylated PBDE metabolites in young humans from Managua, Nicaragua [J].
Athanasiadou, Maria ;
Cuadra, Steven N. ;
Marsh, Goran ;
Bergman, Ake ;
Jakobsson, Kristina .
ENVIRONMENTAL HEALTH PERSPECTIVES, 2008, 116 (03) :400-408
[3]  
Baron E, 2013, CHEMOSPHERE
[4]   Occurrence of hydrophobic organic pollutants (BFRs and UV-filters) in sediments from South America [J].
Baron, Enrique ;
Gago-Ferrero, Pablo ;
Gorga, Marina ;
Rudolph, Ignacio ;
Mendoza, Gonzalo ;
Mauricio Zapata, Andres ;
Diaz-Cruz, Silvia ;
Barra, Ricardo ;
Ocampo-Duque, William ;
Paez, Martha ;
Maria Darbra, Rosa ;
Eljarrat, Ethel ;
Barcelo, Damia .
CHEMOSPHERE, 2013, 92 (03) :309-316
[5]   Polybrominated diphenyl ethers (PBDEs) in Mediterranean mussels (Mytilus galloprovincialis) from selected Apulia coastal sites evaluated by GC-HRMS [J].
Bianco, Giuliana ;
Novario, Giuseppe ;
Anzilotta, Giuseppe ;
Palma, Achille ;
Mangone, Annarosa ;
Cataldi, Tommaso R. I. .
JOURNAL OF MASS SPECTROMETRY, 2010, 45 (09) :1046-1055
[6]   Levels of some polybrominated diphenyl ether (PBDE) flame retardants along the Dutch coast as derived from their accumulation in SPMDs and blue mussels (Mytilus edulis) [J].
Booij, K ;
Zegers, BN ;
Boon, JP .
CHEMOSPHERE, 2002, 46 (05) :683-688
[7]   Biological and chemical factors of importance in the bioaccumulation and trophic transfer of persistent organochlorine contaminants in arctic marine food webs [J].
Borgå, K ;
Fisk, AT ;
Hoekstra, PF ;
Muir, DCG .
ENVIRONMENTAL TOXICOLOGY AND CHEMISTRY, 2004, 23 (10) :2367-2385
[8]   Polybrominated diphenyl ethers (PBDEs) in marine fish and blue mussels from southern Greenland [J].
Christensen, JH ;
Glasius, M ;
Pécseli, M ;
Platz, J ;
Pritzl, G .
CHEMOSPHERE, 2002, 47 (06) :631-638
[9]   Anthropogenic and Naturally Occurring Organobrominated Compounds in Two Deep-Sea Fish Species from the Mediterranean Sea [J].
Covaci, Adrian ;
Losada, Sara ;
Roosens, Laurence ;
Vetter, Walter ;
Javier Santos, Francisco ;
Neels, Hugo ;
Storelli, Arianna ;
Storelli, Maria M. .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2008, 42 (23) :8654-8660
[10]   Novel brominated flame retardants: A review of their analysis, environmental fate and behaviour [J].
Covaci, Adrian ;
Harrad, Stuart ;
Abdallah, Mohamed A. -E. ;
Ali, Nadeem ;
Law, Robin J. ;
Herzke, Dorte ;
de Wit, Cynthia A. .
ENVIRONMENT INTERNATIONAL, 2011, 37 (02) :532-556
123456