In situ plasma-assisted atmospheric nitrogen fixation using water and spray-type jet plasma

被引：71

作者：

Peng, Peng ^{[1
]}

Chen, Paul ^{[1
]}

Addy, Min ^{[1
]}

Cheng, Yanling ^{[1
]}

Zhang, Yaning ^{[1
,2
]}

Anderson, Erik ^{[1
]}

Zhou, Nan ^{[1
]}

Schiappacasse, Charles ^{[1
]}

Hatzenbeller, Raymond ^{[1
]}

Fan, Liangliang ^{[1
]}

Liu, Shiyu ^{[1
]}

Chen, Dongjie ^{[1
]}

Liu, Juer ^{[1
]}

Liu, Yuhuan ^{[3
]}

Ruan, Roger ^{[1
,3
]}

机构：

[1] Univ Minnesota Twin Cities, Dept Bioprod & Biosyst Engn, Ctr Biorefining, St Paul, MN 55108 USA

[2] Harbin Inst Technol, Harbin 150001, Heilongjiang, Peoples R China

[3] Nanchang Univ, MOE Biomass Engn Res Ctr, Nanchang 330047, Jiangxi, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2018年 / 54卷 / 23期

关键词：

PHOTOCHEMICAL DATA; AMMONIA PRODUCTION; GAS; CHEMISTRY; NOX;

D O I：

10.1039/c8cc00697k

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

In this study, a sustainable nitrogen fixation process was presented under atmospheric conditions and without introducing hydrogen or any catalyst. The novel in situ synthesis in this study used an advanced spray-type jet plasma, which significantly improved the fixation rate of nitrite, nitrate, and ammonium. Furthermore, the mechanism focusing on the co-synthesis of the abovementioned three nitrogen compounds was proposed based on the synergistic interactions between the gas-phase plasma and liquid surface dissociation.

引用

页码：2886 / 2889

页数：4

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