Inhomogeneity of donor doping in SrTiO3 substrates studied by fluorescence-lifetime imaging microscopy

被引:14
作者
Rodenbuecher, C. [1 ,2 ]
Gensch, T. [3 ]
Speier, W. [2 ]
Breuer, U. [4 ]
Pilch, M. [1 ,2 ,5 ]
Hardtdegen, H. [2 ,6 ]
Mikulics, M. [2 ,6 ]
Zych, E. [7 ]
Waser, R. [1 ,2 ,8 ]
Szot, K. [1 ,2 ,5 ]
机构
[1] Forschungszentrum Julich, Peter Grunberg Inst PGI 7, D-52425 Julich, Germany
[2] Forschungszentrum Julich, JARA Fundamentals Future Informat Technol, D-52425 Julich, Germany
[3] Forschungszentrum Julich, Inst Complex Syst ICS 4, D-52425 Julich, Germany
[4] Forschungszentrum Julich, Zent Inst Engn Elekt & Analyt ZEA 3, D-52425 Julich, Germany
[5] Univ Silesia, A Chelkowski Inst Phys, PL-40007 Katowice, Poland
[6] Forschungszentrum Julich, Peter Grunberg Inst PGI 9, D-52425 Julich, Germany
[7] Univ Wroclaw, Fac Chem, PL-50383 Wroclaw, Poland
[8] Rhein Westfal TH Aachen, Inst Werkstoffe Elektrotech 2, D-52056 Aachen, Germany
关键词
LIGHT-EMISSION;
D O I
10.1063/1.4825367
中图分类号
O59 [应用物理学];
学科分类号
摘要
Fluorescence-lifetime imaging microscopy (FLIM) was applied to investigate the donor distribution in SrTiO3 single crystals. On the surfaces of Nb- and La-doped SrTiO3, structures with different fluorescence intensities and lifetimes were found that could be related to different concentrations of Ti3+. Furthermore, the inhomogeneous distribution of donors caused a non-uniform conductivity of the surface, which complicates the production of potential electronic devices by the deposition of oxide thin films on top of doped single crystals. Hence, we propose FLIM as a convenient technique (length scale: 1 mu m) for characterizing the quality of doped oxide surfaces, which could help to identify appropriate substrate materials. (C) 2013 AIP Publishing LLC.
引用
收藏
页数:4
相关论文
共 18 条
  • [1] Becker W., 2010, SPRINGER SERIES CHEM, V81
  • [2] 2-PHOTON LASER SCANNING FLUORESCENCE MICROSCOPY
    DENK, W
    STRICKLER, JH
    WEBB, WW
    [J]. SCIENCE, 1990, 248 (4951) : 73 - 76
  • [3] Surface electronic structure of electron-doped SrTiO3
    Haruyama, Y
    Aiura, Y
    Bando, H
    Suzuki, H
    Nishihara, Y
    [J]. PHYSICA B, 1997, 237 : 380 - 382
  • [4] Structure and electrical characteristics of Nb-doped SrTiO3 substrates
    Huang Yanhong
    Lu Huibin
    Guo Haizhong
    Liu Lifeng
    He Meng
    Chen Zhenghao
    Zhou Yueliang
    Zhao Kun
    Jin Kuijuan
    Yang Guozen
    [J]. CHINESE SCIENCE BULLETIN, 2006, 51 (16): : 2035 - 2037
  • [5] Blue luminescence from electron-doped SrTiO3
    Kan, D.
    Kanda, R.
    Kanemitsu, Y.
    Shimakawa, Y.
    Takano, M.
    Terashima, T.
    Ishizumi, A.
    [J]. APPLIED PHYSICS LETTERS, 2006, 88 (19)
  • [6] Blue-light emission at room temperature from Ar+-irradiated SrTiO3
    Kan, DS
    Terashima, T
    Kanda, R
    Masuno, A
    Tanaka, K
    Chu, SC
    Kan, H
    Ishizumi, A
    Kanemitsu, Y
    Shimakawa, Y
    Takano, M
    [J]. NATURE MATERIALS, 2005, 4 (11) : 816 - 819
  • [7] Determination of intracellular chloride concentration in dorsal root ganglion neurons by fluorescence lifetime imaging
    Kaneko, H
    Putzier, V
    Frings, S
    Gensch, T
    [J]. CALCIUM-ACTIVATED CHLORIDE CHANNELS, 2002, 53 : 167 - +
  • [8] Light emission from SrTiO3
    Kanemitsu, Yoshihiko
    Yamada, Yasuhiro
    [J]. PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS, 2011, 248 (02): : 416 - 421
  • [9] Real-time determination of intracellular oxygen in bacteria using a genetically encoded FRET-based biosensor
    Potzkei, Janko
    Kunze, Martin
    Drepper, Thomas
    Gensch, Thomas
    Jaeger, Karl-Erich
    Buechs, Jochen
    [J]. BMC BIOLOGY, 2012, 10
  • [10] Highly conductive nanolayers on strontium titanate produced by preferential ion-beam etching
    Reagor, DW
    Butko, VY
    [J]. NATURE MATERIALS, 2005, 4 (08) : 593 - 596