Numerical investigations on the contribution of point source emissions to the PM2.5 concentrations in Fairbanks, Alaska

被引:7
作者
Tran, Huy N. Q.
Moelders, Nicole [1 ]
机构
[1] Univ Alaska Fairbanks, Inst Geophys, Fairbanks, AK 99775 USA
关键词
WRF/Chem; Point-source emissions; High latitudes; Winter air pollution; PM2.5; PARTICULATE AIR-POLLUTION; MODEL; QUALITY; AEROSOL; WRF/CHEM; PARAMETERIZATION; DEPOSITION; IMPACTS; EUROPE;
D O I
10.5094/APR.2012.022
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Simulations with and without consideration of emissions from point sources were performed with the Weather Research and Forecasting model with online chemistry (WRF/Chem) to examine the contribution of point source emissions to the PM2.5 concentrations at breathing level in Fairbanks, Alaska during winter. On days and at locations where PM2.5 concentrations exceed the National Ambient Air Quality Standard of 35 mu g m(-3), emissions from point sources account for 4% of the 24 h-average PM2.5 concentration on average. The locations of highest concentrations were the same in both simulations. Point source emissions induced only five additional exceedance days in the nonattainment area. The magnitude of the PM2.5 concentrations depended on meteorological conditions (temperature, wind speed, mixing height) and emissions. The radius of impact of point source emissions on the PM2.5 concentration at breathing level of about 10-12 km downwind results as a combination of low emission heights, low wind speeds and the presence of inversions. (C) Author(s) 2012. This work is distributed under the Creative Commons Attribution 3.0 License.
引用
收藏
页码:199 / 210
页数:12
相关论文
共 29 条
  • [1] Modal aerosol dynamics model for Europe: Development and first applications
    Ackermann, IJ
    Hass, H
    Memmesheimer, M
    Ebel, A
    Binkowski, FS
    Shankar, U
    [J]. ATMOSPHERIC ENVIRONMENT, 1998, 32 (17) : 2981 - 2999
  • [2] [Anonymous], 2002, NCEP OFF NOTE
  • [3] Technical Note: Evaluation of the WRF-Chem "Aerosol Chemical to Aerosol Optical Properties" Module using data from the MILAGRO campaign
    Barnard, J. C.
    Fast, J. D.
    Paredes-Miranda, G.
    Arnott, W. P.
    Laskin, A.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2010, 10 (15) : 7325 - 7340
  • [4] Asian aerosol transport to Alaska during ACE-Asia
    Cahill, CF
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2003, 108 (D23)
  • [5] Coupling aerosol-cloud-radiative processes in the WRF-Chem model: Investigating the radiative impact of elevated point sources
    Chapman, E. G.
    Gustafson, W. I., Jr.
    Easter, R. C.
    Barnard, J. C.
    Ghan, S. J.
    Pekour, M. S.
    Fast, J. D.
    [J]. ATMOSPHERIC CHEMISTRY AND PHYSICS, 2009, 9 (03) : 945 - 964
  • [6] The assessment of emission-source contributions to air quality by using a coupled MM5-ARPS-CMAQ modeling system: A case study in the Beijing metropolitan region, China
    Cheng, Shuiyuan
    Chen, Dongsheng
    Li, Jianbing
    Wang, Haiyan
    Guo, Xiurui
    [J]. ENVIRONMENTAL MODELLING & SOFTWARE, 2007, 22 (11) : 1601 - 1616
  • [7] Chou M. D., 1994, EFFICIENT THERMAL IN
  • [8] Fine particulate air pollution and hospital admission for cardiovascular and respiratory diseases
    Dominici, F
    Peng, RD
    Bell, ML
    Pham, L
    McDermott, A
    Zeger, SL
    Samet, JM
    [J]. JAMA-JOURNAL OF THE AMERICAN MEDICAL ASSOCIATION, 2006, 295 (10): : 1127 - 1134
  • [9] Effects of changing power plant NOx emissions on ozone in the eastern United States:: Proof of concept
    Frost, G. J.
    McKeen, S. A.
    Trainer, M.
    Ryerson, T. B.
    Neuman, J. A.
    Roberts, J. M.
    Swanson, A.
    Holloway, J. S.
    Sueper, D. T.
    Fortin, T.
    Parrish, D. D.
    Fehsenfeld, F. C.
    Flocke, F.
    Peckham, S. E.
    Grell, G. A.
    Kowal, D.
    Cartwright, J.
    Auerbach, N.
    Habermann, T.
    [J]. JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2006, 111 (D12)
  • [10] Fully coupled "online" chemistry within the WRF model
    Grell, GA
    Peckham, SE
    Schmitz, R
    McKeen, SA
    Frost, G
    Skamarock, WC
    Eder, B
    [J]. ATMOSPHERIC ENVIRONMENT, 2005, 39 (37) : 6957 - 6975