Artificial neural networks with response surface methodology for optimization of selective CO2 hydrogenation using K-promoted iron catalyst in a microchannel reactor

被引:53
|
作者
Sun, Yong [1 ]
Yang, Gang [2 ]
Wen, Chao [3 ]
Zhang, Lian [4 ]
Sun, Zhi [5 ]
机构
[1] Edith Cowan Univ, Sch Engn, 270 Joondalup Dr, Joondalup, WA 6027, Australia
[2] Anpeng High Tech Energy Corp, Beijing, Peoples R China
[3] Northwest Univ, Res Ctr Intelligent Interact & Informat Art, Xian 710069, Shaanxi, Peoples R China
[4] Monash Univ, Dept Chem Engn, Clayton, Vic 3800, Australia
[5] Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Beijing 100190, Peoples R China
关键词
ANNs/RSM; Optimization; CO2; hydrogenation; Iron-based catalyst; Microchannel reactor; FISCHER-TROPSCH SYNTHESIS; PRODUCT DISTRIBUTION; ACTIVATED CARBON; OPERATING-CONDITIONS; LIQUID PRODUCTS; LIGHT OLEFINS; REMOVAL; ANNS; RSM; PERFORMANCE;
D O I
10.1016/j.jcou.2017.11.013
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
CO2 hydrogenation was optimized by a combination of AANs (Artificial Neuron Networks) with RSM (Response Surface Methodology) in a microchannel reactor using a K-promoted iron-based catalyst. This robust and cost-effective methodology was reliable to extensively analyze the effect of operating conditions i.e. gas ratio, temperature, pressure, and space velocity on product distribution of selective CO2 hydrogenation. With experimental data as training data using ANNs and Box-Behnken design as design of experiment, the obtained model was able to present good results in a nonlinear noisy process with significant changes of critical operation parameters in an experimental design plan during CO2 hydrogenation using K-promoted iron-based catalyst in a microchannel reactor. The achieved quadratic model was flexible and effective in optimizing either single or multiple objections of product distribution for CO2 hydrogenation.
引用
收藏
页码:10 / 21
页数:12
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