A review of linear carbon chains

被引：65
作者：
Zhang, Kan [1 ]
Zhang, Yifan [1 ]
Shi, Lei [1 ]
机构：
[1] Sun Yat Sen Univ, Sch Mat Sci & Engn, Nanotechnol Res Ctr, State Key Lab Optoelect Mat & Technol, Guangzhou 510275, Peoples R China
来源：
CHINESE CHEMICAL LETTERS | 2020年 / 31卷 / 07期
基金：
中国国家自然科学基金;
关键词：
Linear carbon chains; Polyyne; Carbyne; Carbon nanotubes; Electronic property; BOND-LENGTH ALTERNATION; HYDROGEN-CAPPED POLYYNES; LASER-ABLATION; ACETYLENIC-COMPOUNDS; RAMAN-SPECTROSCOPY; BAND-STRUCTURE; HARTREE-FOCK; VIBRATIONAL PROPERTIES; ELECTRONIC-PROPERTIES; OPTICAL-PROPERTIES;
D O I：
10.1016/j.cclet.2020.03.019
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
Linear carbon chains (LCCs) are a one-dimensional sp(1)-hybridized allotrope of carbon. LCCs are extremely unstable: The longer the LCCs, the less stable the materials. Thus, it is a big challenge to synthesize long LCCs. Although the research on the short LCCs, e.g., polyynes, can be traced back to the 18th, LCCs are still not well-known compared to other allotropes of carbon, e.g., fullerenes, carbon nanotubes and graphene. Therefore, introducing recent progress on LCCs is of great significance to draw more attention in the community of nanocarbons as well as nanomaterials in general. Theoretically, various excellent properties have been predicted. Experimentally, LCCs with different length in many kinds of forms have been successfully synthesized. In this review, we summarized recent studies of polyynic LCCs from both theoretical and experimental aspects. Also, perspectives are highlighted to point out the further investigations of the materials. (C) 2020 Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences. Published by Elsevier B.V. All rights reserved.
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收藏
页码：1746 / 1756
页数：11
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