Spin-State Crossover Model for the Magnetism of Iron Pnictides

被引:26
作者
Chaloupka, Jiri [1 ,2 ]
Khaliullin, Giniyat [1 ]
机构
[1] Max Planck Inst Solid State Res, D-70569 Stuttgart, Germany
[2] Masaryk Univ, Cent European Inst Technol, CS-61137 Brno, Czech Republic
基金
欧盟第七框架计划;
关键词
EXCITATIONS;
D O I
10.1103/PhysRevLett.110.207205
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We propose a minimal model describing magnetic behavior of Fe-based superconductors. The key ingredient of the model is a dynamical mixing of quasidegenerate spin states of Fe2+ ion by intersite electron hoppings, resulting in an effective local spin S-eff. The moments S-eff tend to form singlet pairs and may condense into a spin nematic phase due to the emergent biquadratic exchange couplings. The long-range ordered part m of S-eff varies widely, 0 <= m <= S-eff, but magnon spectra are universal and scale with S-eff, resolving the puzzle of large but fluctuating Fe moments. Unusual temperature dependences of a local moment and spin susceptibility are also explained.
引用
收藏
页数:5
相关论文
共 43 条
[1]   Magnetism, superconductivity, and pairing symmetry in iron-based superconductors [J].
Chubukov, A. V. ;
Efremov, D. V. ;
Eremin, I. .
PHYSICAL REVIEW B, 2008, 78 (13)
[2]   Iron pnictides as a new setting for quantum criticality [J].
Dai, Jianhui ;
Si, Qimiao ;
Zhu, Jian-Xin ;
Abrahams, Elihu .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2009, 106 (11) :4118-4121
[3]   Spinor bosonic atoms in optical lattices: Symmetry breaking and fractionalization [J].
Demler, E ;
Zhou, F .
PHYSICAL REVIEW LETTERS, 2002, 88 (16) :4
[4]   Theory of electron nematic order in LaFeAsO [J].
Fang, Chen ;
Yao, Hong ;
Tsai, Wei-Feng ;
Hu, JiangPing ;
Kivelson, Steven A. .
PHYSICAL REVIEW B, 2008, 77 (22)
[5]   Near-degeneracy of several pairing channels in multiorbital models for the Fe pnictides [J].
Graser, S. ;
Maier, T. A. ;
Hirschfeld, P. J. ;
Scalapino, D. J. .
NEW JOURNAL OF PHYSICS, 2009, 11
[6]   Spin-State Transition in the Fe Pnictides [J].
Gretarsson, H. ;
Saha, S. R. ;
Drye, T. ;
Paglione, J. ;
Kim, Jungho ;
Casa, D. ;
Gog, T. ;
Wu, W. ;
Julian, S. R. ;
Kim, Young-June .
PHYSICAL REVIEW LETTERS, 2013, 110 (04)
[7]   Revealing the dual nature of magnetism in iron pnictides and iron chalcogenides using x-ray emission spectroscopy [J].
Gretarsson, H. ;
Lupascu, A. ;
Kim, Jungho ;
Casa, D. ;
Gog, T. ;
Wu, W. ;
Julian, S. R. ;
Xu, Z. J. ;
Wen, J. S. ;
Gu, G. D. ;
Yuan, R. H. ;
Chen, Z. G. ;
Wang, N. -L. ;
Khim, S. ;
Kim, K. H. ;
Ishikado, M. ;
Jarrige, I. ;
Shamoto, S. ;
Chu, J. -H. ;
Fisher, I. R. ;
Kim, Young-June .
PHYSICAL REVIEW B, 2011, 84 (10)
[8]   Spin crossover -: An overall perspective [J].
Gütlich, P ;
Goodwin, HA .
SPIN CROSSOVER IN TRANSITION METAL COMPOUNDS I, 2004, 233 :1-47
[9]   Quadrupolar order in isotropic Heisenberg models with biquadratic interaction [J].
Harada, K ;
Kawashima, N .
PHYSICAL REVIEW B, 2002, 65 (05) :1-4
[10]   Spin-exchange interactions of spin-one bosons in optical lattices: Singlet, nematic, and dimerized phases [J].
Imambekov, A ;
Lukin, M ;
Demler, E .
PHYSICAL REVIEW A, 2003, 68 (06) :24