Influence of the embedding matrix on optical properties of Ge nanocrystals-based nanocomposite

被引:10
作者
Parola, S. [1 ]
Quesnel, E. [1 ]
Muffato, V. [1 ]
Bartringer, J. [2 ]
Slaoui, A. [2 ]
机构
[1] CEA G DRT LITEN DTNM, F-38054 Grenoble 9, France
[2] InESS CNRS UMR 7163, F-67037 Strasbourg 2, France
关键词
SILICON QUANTUM DOTS; GERMANIUM NANOCRYSTALS; PHOTOLUMINESCENCE; FILMS; CONFINEMENT; EXCITONS; AL2O3; CELLS;
D O I
10.1063/1.4789959
中图分类号
O59 [应用物理学];
学科分类号
摘要
Germanium nanocrystals were prepared by a nanocluster source and characterized by photoluminescence and spectroscopic photometry methods. The optical measurements were carried out in order to estimate the effective bandgap of the Ge nanocrystals. Both Mie theory and the quantum confinement theory were applied to interpret the extracted absorption data. We found that the quantum confinement theory enables to explain the nanocrystal size and the host matrix dependence of the nanocrystal bandgap. On the other hand, the photoluminescence measurements have not allowed to confirm the bandgap evaluated from absorption data. This is explained as due to the dominant effect of the recombination at the nanocrystals surface. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789959]
引用
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页数:8
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共 30 条
  • [11] Optical gap of silicon crystallites embedded in various wide-band amorphous matrices: role of environment
    Konakov, A. A.
    Burdov, V. A.
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2010, 22 (21)
  • [12] Exciton states and photoluminescence of silicon and germanium nanocrystals in an Al2O3 matrix
    Kupchak, I. M.
    Kryuchenko, Yu. V.
    Korbutyak, D. V.
    Sachenko, A. V.
    Kaganovich, E. B.
    Manoilov, E. G.
    Begun, E. V.
    [J]. SEMICONDUCTORS, 2008, 42 (10) : 1194 - 1199
  • [13] Structural and optical study of Ge nanocrystals embedded in Si3N4 matrix
    Lee, S.
    Huang, S.
    Conibeer, G.
    Green, M. A.
    [J]. EUROPEAN MATERIALS RESEARCH SOCIETY CONFERENCE SYMPOSIUM: ADVANCED INORGANIC MATERIALS AND CONCEPTS FOR PHOTOVOLTAICS, 2011, 10
  • [14] Wavelength dependent photoluminescence of anodic alumina membranes
    Li, GH
    Zhang, Y
    Wu, YC
    Zhang, LD
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 2003, 15 (49) : 8663 - 8671
  • [15] Quantum confinement in germanium nanocrystals
    Niquet, YM
    Allan, G
    Delerue, C
    Lannoo, M
    [J]. APPLIED PHYSICS LETTERS, 2000, 77 (08) : 1182 - 1184
  • [16] n-Type silicon quantum dots and p-type crystalline silicon heteroface solar cells
    Park, Sangwook
    Cho, Eunchel
    Song, Dengyuan
    Conibeer, Gavin
    Green, Martin A.
    [J]. SOLAR ENERGY MATERIALS AND SOLAR CELLS, 2009, 93 (6-7) : 684 - 690
  • [17] Parola S., 2010, Proceedings of the 25th European Photovoltaic Solar Energy Conference and Exhibition and the 5th World Conference on Photovoltaic Energy Conversion, P622
  • [18] Structural properties of Ge nanocrystals synthesized by a PVD nanocluster source
    Parola, S.
    Quesnel, E.
    Muffato, V.
    Guetaz, L.
    Szambolics, H.
    Bartringer, J.
    Slaoui, A.
    [J]. JOURNAL OF NANOPARTICLE RESEARCH, 2012, 14 (09)
  • [19] Modeling metallic nanoparticle synthesis in a magnetron-based nanocluster source by gas condensation of a sputtered vapor
    Quesnel, E.
    Pauliac-Vaujour, E.
    Muffato, V.
    [J]. JOURNAL OF APPLIED PHYSICS, 2010, 107 (05)
  • [20] Photoluminescence mechanisms in silicon quantum dots embedded in nanometric chlorinated-silicon nitride films
    Rodriguez, A.
    Arenas, J.
    Alonso, J. C.
    [J]. JOURNAL OF LUMINESCENCE, 2012, 132 (09) : 2385 - 2389