Experimental method for simultaneous and continuous measurement of absorption rate, viscosity and heat of reaction of carbon dioxide capture solvents

被引:6
作者
Kim, Junghwan [1 ]
Kim, Huiyong [1 ]
Kim, Jayeop [1 ]
Hwang, Sung June [1 ]
Lee, Kwang Soon [1 ]
机构
[1] Sogang Univ, Chem & Biomol Engn Dept, 35 Baekbeom Ro, Seoul 121742, South Korea
关键词
Carbon dioxide capture; Solvent screening; Wetted wall column; Simultaneous measurements; Continuous measurements; AQUEOUS AMINE SOLUTIONS; STOPPED-FLOW TECHNIQUE; CO2; ABSORPTION; MONOETHANOLAMINE MEA; KINETICS;
D O I
10.1016/j.jiec.2017.12.012
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
When screening solvents for carbon capture, a large amount of property data for each solvent in the CO2-loaded state is required. In this paper, a novel experimental method is proposed that involves modifying a wetted wall column in order to simultaneously measure the absorption rate, viscosity, pH, and heat of reaction of carbon capture solvents while the CO2 loading is increased continuously. The proposed method was applied to 30 wt% aqueous monoethanolamine and 30 wt% aqueous piperazine as solvents and found to produce measurement results that matched well with literature data. (C) 2017 Published by Elsevier B.V. on behalf of The Korean Society of Industrial and Engineering Chemistry.
引用
收藏
页码:152 / 160
页数:9
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