Revisiting the collision-induced light scattering spectrum of gaseous CH4

被引：0
|
作者：
Meinander, N
Tabisz, GC
Barocchi, F
Zoppi, M
机构：
[1] UNIV MANITOBA, DEPT PHYS, WINNIPEG, MB R3T 2N2, CANADA
[2] UNIV FLORENCE, DIPARTIMENTO FIS, I-50125 FLORENCE, ITALY
[3] CNR, IST ELETTRON QUANTIST, I-50127 FLORENCE, ITALY
来源：
MOLECULAR PHYSICS | 1996年 / 89卷 / 02期
关键词：
D O I：
10.1080/002689796173886
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
The profile of the two-body collision-induced light scattering spectrum of CH4 at temperatures from 295 K to 130 K is calculated through a classical trajectory simulation of the collision. Free translational, bound state, and single and double induced rotational contributions are included. The magnitudes of the dipole-quadrupole and dipole-octopole polarizabilities are found to be 0.75 Angstrom(4) and 2.7 Angstrom(5), respectively, through comparison with experiment.
引用
收藏
页码：521 / 531
页数：11
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