Thermal conductance of an individual single-wall carbon nanotube above room temperature

被引:1435
作者
Pop, E
Mann, D
Wang, Q
Goodson, KE
Dai, HJ [1 ]
机构
[1] Stanford Univ, Dept Chem, Stanford, CA 94305 USA
[2] Stanford Univ, Lab Adv Mat, Stanford, CA 94305 USA
[3] Stanford Univ, Dept Mech Engn & Thermal Sci, Stanford, CA 94305 USA
关键词
D O I
10.1021/nl052145f
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The thermal properties of a suspended metallic single-wall carbon nanotube (SWNT) are extracted from its high-bias (l-V) electrical characteristics over the 300-800 K temperature range, achieved by Joule self-heating. The thermal conductance is approximately 2.4 nW/K, and the thermal-conductivity is nearly 3500 Wm(-1)K(-1) at room temperature for a SWNT of length 2.6 mu m and diameter 1.7 nm. A subtle decrease in thermal conductivity steeper than 1/T is observed at the upper end of the temperature range, which is attributed to second-order three-phonon scattering between two acoustic modes and one optical mode. We discuss sources of uncertainty and propose a simple analytical model for the SWNT thermal conductivity including length and temperature dependence.
引用
收藏
页码:96 / 100
页数:5
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