Compositional and Interface Engineering of Organic-Inorganic Lead Halide Perovskite Solar Cells

被引:143
作者
Lu, Haizhou [1 ,2 ]
Krishna, Anurag [1 ]
Zakeeruddin, Shaik M. [2 ]
Gratzel, Michael [2 ]
Hagfeldt, Anders [1 ]
机构
[1] Ecole Polytech Fed Lausanne EPFL, Lab Photomol Sci, Inst Chem Sci Engn, CH-1015 Lausanne, Switzerland
[2] Ecole Polytech Fed Lausanne EPFL, Lab Photon & Interfaces, Inst Chem Sci & Engn, CH-1015 Lausanne, Switzerland
基金
瑞士国家科学基金会; 欧盟地平线“2020”;
关键词
HIGH-EFFICIENCY; DEFECT PASSIVATION; PERFORMANCE; IODIDE; PHOTOLUMINESCENCE; MANAGEMENT; STABILITY; TRIHALIDE; BANDGAP; LENGTHS;
D O I
10.1016/j.isci.2020.101359
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Power conversion efficiency (PCE) of the perovskite solar cells (PSCs) has remark-ably been increased from 3.1% to 25.2%. The fast expansion of the PSCs has been along with the development of compositional and interface engineering, which has been playing a critical role. For the PSCs with record high-efficiency and sta-bility, the perovskite absorber layer has been changed from the initial MAPbI(3)- to FAPbI(3)-based compositions. Owing to the enormous engineering works, perov-skite absorber layers with monolithic grains could be achieved, in which the interior defects are negligible compared with the surface defects. Therefore, interface engineering, which can passivate the surface defects and/or isolate the perovskite from the environmental moistures, has been playing a more and more important role to further boost the PCE and stability of the PSCs. Herein, a compact review study of the compositional and interface engineering is pre-sented and promising strategies and directions of the PSCs are discussed.
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页数:14
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