Bimetallic Aerogels: High-Performance Electrocatalysts for the Oxygen Reduction Reaction

被引:238
作者
Liu, Wei [1 ]
Rodriguez, Paramaconi [2 ,3 ]
Borchardt, Lars [1 ]
Foelske, Annette [2 ]
Yuan, Jipei [1 ]
Herrmann, Anne-Kristin [1 ]
Geiger, Dorin [4 ]
Zheng, Zhikun [5 ]
Kaskel, Stefan [1 ]
Gaponik, Nikolai [1 ]
Koetz, Ruediger [2 ]
Schmidt, Thomas J. [2 ]
Eychmueller, Alexander [1 ]
机构
[1] Tech Univ Dresden, D-01062 Dresden, Germany
[2] Paul Scherrer Inst, Electrochem Lab, CH-5232 Villigen, Switzerland
[3] Univ Birmingham, Sch Chem, Birmingham B15 2TT, W Midlands, England
[4] Tech Univ Dresden, Inst Struct Phys, Triebenberg Lab HRTEM & Electron Holog, D-01328 Dresden, Germany
[5] ETH, Inst Polymere, CH-8093 Zurich, Switzerland
关键词
aerogels; electrocatalysis; oxygen reduction reaction; palladium; platinum; ELECTROLYTE FUEL-CELLS; PLATINUM NANOPARTICLES; METAL FOAMS; CATALYSTS; SIZE; CHALLENGES; CLUSTERS;
D O I
10.1002/anie.201303109
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Best of both worlds: PtxPdy, Pt, and Pd aerogels with high surface area and porosity can be synthesized in a controlled fashion by a straightforward and environmentally benign strategy. These materials, which are highly active and stable catalysts for the oxygen reduction reaction in PEFC cathodes, combine the high stability of extended surfaces with the high surface area of nanoparticles. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:9849 / 9852
页数:4
相关论文
共 41 条
[1]  
[Anonymous], 2009, ANGEW CHEM INT ED, V48, P9731
[2]  
[Anonymous], 2010, ANGEW CHEM INT ED, V49, P4544
[3]  
[Anonymous], 2008, ANGEW CHEM INT ED, V47, P3588
[4]  
[Anonymous], 2012, ANGEW CHEM INT ED, V51, P5743
[5]  
[Anonymous], 2006, ANGEW CHEM-GER EDIT, DOI DOI 10.1002/ANGE.200504386
[6]  
[Anonymous], 2012, ANGEW CHEM INT ED, V51, P4641
[7]  
[Anonymous], 2011, ANGEW CHEM INT ED, V50, P6346
[8]  
[Anonymous], 2006, ANGEW CHEM INT ED, V45, P2897
[9]   Rational synthesis of Pt spheres with hollow interior and nanosponge shell using silica particles as template [J].
Ataee-Esfahani, Hamed ;
Nemoto, Yoshihiro ;
Wang, Liang ;
Yamauchi, Yusuke .
CHEMICAL COMMUNICATIONS, 2011, 47 (13) :3885-3887
[10]  
Bigall N. C., 2009, ANGEW CHEM, V121, P9911