Interface Engineering of electron Transport Layer-Free Planar Perovskite Solar Cells with Efficiency Exceeding 15%

被引:13
作者
Huang, Feiyue [1 ,3 ]
Wei, Yuelin [1 ,3 ]
Gu, Lin [1 ,3 ]
Guo, Qiyao [1 ,3 ]
Xu, Hui [2 ,3 ]
Luo, Dan [2 ,3 ]
Jin, Shao [1 ,3 ]
Yang, Xiaomin [1 ,3 ]
Huang, Yunfang [2 ,3 ]
Wu, Jihuai [1 ,3 ]
机构
[1] Huaqiao Univ, Coll Mat Sci & Engn, Xiamen 361021, Peoples R China
[2] Huaqiao Univ, Coll Chem Engn, Xiamen 361021, Peoples R China
[3] Huaqiao Univ, Minist Educ, Engn Res Ctr Environm Friendly Funct Mat, Xiamen 361021, Peoples R China
基金
美国国家科学基金会; 中国国家自然科学基金;
关键词
electron transport layer; perovskite solar cell; plasma cleaning; power conversion efficiency; COMPACT LAYER; TIN OXIDE; PERFORMANCE; TEMPERATURE; EXTRACTION; DEPOSITION;
D O I
10.1002/ente.201700437
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
A high-performance electron transport layer (ETL)-free planar fluorine-doped tin oxide (FTO)/perovskite/hole-transport material/Au solar cell was prepared. We revealed that a plasma-cleaning pretreatment for FTO substrates could significantly improve the quality of perovskite films, leading to the promotion of charge separation, an increase in the elec-tron-transport rate, and a decrease in the recombination reaction at the FTO/perovskite interface. Finally, the efficiency of the cells was greatly improved. A power conversion efficiency of over 15% and a fill factor of 0.68 were achieved under AM 1.5G 100 mW cm(-2) irradiation without the use of a compact n-type metal-oxide blocking layer.
引用
收藏
页码:1844 / 1851
页数:8
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