Electron Transfer and Ionic Displacements as the Origin of the 2D Electron Gas at the LAO/STO Interface: Direct Measurements with Atomic-Column Spatial Resolution

被引:134
作者
Cantoni, Claudia [1 ]
Gazquez, Jaume [1 ,2 ]
Granozio, Fabio Miletto [3 ,4 ]
Oxley, Mark P. [1 ]
Varela, Maria [1 ]
Lupini, Andrew R. [1 ]
Pennycook, Stephen J. [1 ]
Aruta, Carmela [3 ,4 ]
di Uccio, Umberto Scotti [3 ,4 ]
Perna, Paolo [3 ,4 ]
Maccariello, Davide [3 ,4 ]
机构
[1] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA
[2] Univ Complutense Madrid, E-28040 Madrid, Spain
[3] Univ Naples Federico II, Dipartimento Sci Fis, I-80126 Naples, Italy
[4] Univ Naples Federico II, CNR SPIN, I-80126 Naples, Italy
基金
欧洲研究理事会;
关键词
TRANSITION-METAL OXIDES; NEAR-EDGE STRUCTURES; X-RAY-ABSORPTION; SRTIO3/LAALO3; INTERFACES; CONDUCTIVITY; SPECTRA; CHARGE; SRTIO3;
D O I
10.1002/adma.201200667
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Using state-of-the-art, aberration-corrected scanning transmission electron microscopy and electron energy loss spectroscopy with atomic-scale spatial resolution, experimental evidence for an intrinsic electronic reconstruction at the LAO/STO interface is shown. Simultaneous measurements of interfacial electron density and system polarization are crucial for establishing the highly debated origin of the 2D electron gas. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:3952 / 3957
页数:6
相关论文
共 38 条
[1]   SOFT-X-RAY-ABSORPTION STUDIES OF THE LOCATION OF EXTRA CHARGES INDUCED BY SUBSTITUTION IN CONTROLLED-VALENCE MATERIALS [J].
ABBATE, M ;
DEGROOT, FMF ;
FUGGLE, JC ;
FUJIMORI, A ;
TOKURA, Y ;
FUJISHIMA, Y ;
STREBEL, O ;
DOMKE, M ;
KAINDL, G ;
VANELP, J ;
THOLE, BT ;
SAWATZKY, GA ;
SACCHI, M ;
TSUDA, N .
PHYSICAL REVIEW B, 1991, 44 (11) :5419-5422
[2]   Pulsed laser deposition of SrTiO3/LaGaO3 and SrTiO3/LaAlO3: Plasma plume effects [J].
Aruta, C. ;
Amoruso, S. ;
Bruzzese, R. ;
Wang, X. ;
Maccariello, D. ;
Granozio, F. Miletto ;
di Uccio, U. Scotti .
APPLIED PHYSICS LETTERS, 2010, 97 (25)
[3]   ELECTRON ENERGY-LOSS NEAR-EDGE STRUCTURES AT THE OXYGEN K-EDGES OF TITANIUM(IV) OXYGEN COMPOUNDS [J].
BRYDSON, R ;
SAUER, H ;
ENGEL, W ;
HOFER, F .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1992, 4 (13) :3429-3437
[4]   Electrostriction at the LaAlO3/SrTiO3 Interface [J].
Cancellieri, C. ;
Fontaine, D. ;
Gariglio, S. ;
Reyren, N. ;
Caviglia, A. D. ;
Fete, A. ;
Leake, S. J. ;
Pauli, S. A. ;
Willmott, P. R. ;
Stengel, M. ;
Ghosez, Ph. ;
Triscone, J. -M. .
PHYSICAL REVIEW LETTERS, 2011, 107 (05)
[5]   Nanoscale control of an interfacial metal-insulator transition at room temperature [J].
Cen, C. ;
Thiel, S. ;
Hammerl, G. ;
Schneider, C. W. ;
Andersen, K. E. ;
Hellberg, C. S. ;
Mannhart, J. ;
Levy, J. .
NATURE MATERIALS, 2008, 7 (04) :298-302
[6]   Instability, intermixing and electronic structure at the epitaxial LaAlO3/SrTiO3(001) heterojunction [J].
Chambers, S. A. ;
Engelhard, M. H. ;
Shutthanandan, V. ;
Zhu, Z. ;
Droubay, T. C. ;
Qiao, L. ;
Sushko, P. V. ;
Feng, T. ;
Lee, H. D. ;
Gustafsson, T. ;
Garfunkel, E. ;
Shah, A. B. ;
Zuo, J-M ;
Ramasse, Q. M. .
SURFACE SCIENCE REPORTS, 2010, 65 (10-12) :317-352
[7]   Understanding the mechanism of conductivity at the LaAlO3/SrTiO3(001) interface [J].
Chambers, Scott A. .
SURFACE SCIENCE, 2011, 605 (13-14) :1133-1140
[8]   Electronic and Magnetic Properties of SrTiO3/LaAlO3 Interfaces from First Principles [J].
Chen, Hanghui ;
Kolpak, Alexie M. ;
Ismail-Beigi, Sohrab .
ADVANCED MATERIALS, 2010, 22 (26-27) :2881-2899
[9]   OXYGEN 1S X-RAY-ABSORPTION EDGES OF TRANSITION-METAL OXIDES [J].
DEGROOT, FMF ;
GRIONI, M ;
FUGGLE, JC ;
GHIJSEN, J ;
SAWATZKY, GA ;
PETERSEN, H .
PHYSICAL REVIEW B, 1989, 40 (08) :5715-5723
[10]  
Egerton R.F., 1996, ELECT ENERGY LOSS SP