Conjugated Polymer Nanomaterials for Solar Water Splitting

被引:65
作者
Dai, Chunhui [1 ]
Pan, Yutong [2 ]
Liu, Bin [2 ,3 ]
机构
[1] East China Univ Technol, Jiangxi Key Lab Mass Spectrometry & Instrumentat, Nanchang 330013, Jiangxi, Peoples R China
[2] Natl Univ Singapore, Dept Chem & Biomol Engn, 4 Engn Dr 4, Singapore 117585, Singapore
[3] Tianjin Univ, Joint Sch Natl Univ Singapore & Tianjin Univ, Int Campus, Fuzhou 350207, Peoples R China
基金
新加坡国家研究基金会; 美国国家科学基金会;
关键词
conjugated polymers; nanomaterials; solar water splitting; CARBON NITRIDE NANOSHEETS; HYDROGEN-PRODUCTION; PHOTOCATALYSTS; EVOLUTION; REDUCTION; NANORODS; DOTS;
D O I
10.1002/aenm.202002474
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Exploration of robust and inexpensive photocatalysts for direct water splitting is highly desirable for solar energy utilization but remains a great challenge. Although some inorganic semiconductors have shown very promising activities, many suffer from low quantum efficiency and insufficient sunlight absorption or present environmental hazards. In recent years, conjugated polymer nanomaterials have rapidly become one of the most appealing candidates in photocatalysis, owing to their facile molecular functionalization, tunable optoelectronic properties, and good chemical stability. This essay highlights the recent advancement of conjugated polymer nanomaterials for solar water splitting. The research opportunities related to water photolysis together with the perspective and challenges in the field are discussed to inspire further exciting research in water splitting.
引用
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页数:8
相关论文
共 44 条
[21]   Semiconductor polymeric graphitic carbon nitride photocatalysts: the "holy grail" for the photocatalytic hydrogen evolution reaction under visible light [J].
Liao, Guangfu ;
Gong, Yan ;
Zhang, Li ;
Gao, Haiyang ;
Yang, Guan-Jun ;
Fang, Baizeng .
ENERGY & ENVIRONMENTAL SCIENCE, 2019, 12 (07) :2080-2147
[22]   Crystalline Carbon Nitride Semiconductors for Photocatalytic Water Splitting [J].
Lin, Lihua ;
Yu, Zhiyang ;
Wang, Xinchen .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2019, 58 (19) :6164-6175
[23]   Metal-free efficient photocatalyst for stable visible water splitting via a two-electron pathway [J].
Liu, Juan ;
Liu, Yang ;
Liu, Naiyun ;
Han, Yuzhi ;
Zhang, Xing ;
Huang, Hui ;
Lifshitz, Yeshayahu ;
Lee, Shuit-Tong ;
Zhong, Jun ;
Kang, Zhenhui .
SCIENCE, 2015, 347 (6225) :970-974
[24]   Synthesis of Sulfur-Doped 2D Graphitic Carbon Nitride Nanosheets for Efficient Photocatalytic Degradation of Phenol and Hydrogen Evolution [J].
Lv, Haiqin ;
Huang, Ying ;
Koodali, Ranjit T. ;
Liu, Guimei ;
Zeng, Yubin ;
Meng, Qingguo ;
Yuan, Mingzhe .
ACS APPLIED MATERIALS & INTERFACES, 2020, 12 (11) :12656-12667
[25]   EFFICIENT VISIBLE-LIGHT-DRIVEN PHOTOCATALYSIS - POLY(PYRIDINE-2,5-DIYL)-CATALYZED HYDROGEN PHOTOEVOLUTION AND PHOTOREDUCTION OF CARBONYL-COMPOUNDS [J].
MATSUOKA, S ;
KOHZUKI, T ;
NAKAMURA, A ;
PAC, C ;
YANAGIDA, S .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1991, (08) :580-581
[26]   Graphitic carbon nitride (g-C3N4)-based metal-free photocatalysts for water splitting: A review [J].
Mishra, Amit ;
Mehta, Akansha ;
Basu, Soumen ;
Shetti, Nagaraj P. ;
Reddy, Kakarla Raghava ;
Aminabhavi, Tejraj M. .
CARBON, 2019, 149 (693-721) :693-721
[27]   Graphitic Carbon Nitride (g-C3N4)-Based Photocatalysts for Artificial Photosynthesis and Environmental Remediation: Are We a Step Closer To Achieving Sustainability? [J].
Ong, Wee-Jun ;
Tan, Lling-Lling ;
Ng, Yun Hau ;
Yong, Siek-Ting ;
Chai, Siang-Piao .
CHEMICAL REVIEWS, 2016, 116 (12) :7159-7329
[28]   An experimental and theoretical study of an efficient polymer nano-photocatalyst for hydrogen evolution [J].
Pati, Palas Baran ;
Damas, Giane ;
Tian, Lei ;
Fernandes, Daniel L. A. ;
Zhang, Lei ;
Pehlivan, Ilknur Bayrak ;
Edvinsson, Tomas ;
Araujo, C. Moyses ;
Tian, Haining .
ENERGY & ENVIRONMENTAL SCIENCE, 2017, 10 (06) :1372-1376
[29]   Metal-free photocatalysts for hydrogen evolution [J].
Rahman, Mohammad Ziaur ;
Kibria, Md Golam ;
Mullins, Charles Buddie .
CHEMICAL SOCIETY REVIEWS, 2020, 49 (06) :1887-1931
[30]   NOVEL VISIBLE-LIGHT-DRIVEN PHOTOCATALYST - POLY(PARA-PHENYLENE)-CATALYZED PHOTOREDUCTIONS OF WATER, CARBONYL-COMPOUNDS, AND OLEFINS [J].
SHIBATA, T ;
KABUMOTO, A ;
SHIRAGAMI, T ;
ISHITANI, O ;
PAC, C ;
YANAGIDA, S .
JOURNAL OF PHYSICAL CHEMISTRY, 1990, 94 (05) :2068-2076