Ba8CoNb6O24: A spin-1/2 triangular-lattice Heisenberg antiferromagnet in the two-dimensional limit

被引:50
作者
Rawl, R. [1 ]
Ge, L. [2 ]
Agrawal, H. [3 ]
Kamiya, Y. [4 ]
Dela Cruz, C. R. [3 ]
Butch, N. P. [5 ]
Sun, X. F. [6 ,7 ,8 ]
Lee, M. [9 ,10 ]
Choi, E. S. [10 ]
Oitmaa, J. [11 ]
Batista, C. D. [1 ,3 ,12 ]
Mourigal, M. [2 ]
Zhou, H. D. [1 ,10 ]
Ma, J. [1 ,8 ,13 ]
机构
[1] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA
[2] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA
[3] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37381 USA
[4] RIKEN, Condensed Matter Theory Lab, Wako, Saitama 3510198, Japan
[5] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA
[6] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China
[7] Chinese Acad Sci, Key Lab Strongly Coupled Quantum Matter Phys, Anhua 230026, Peoples R China
[8] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China
[9] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA
[10] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
[11] Univ New South Wales, Sch Phys, Sydney, NSW 2052, Australia
[12] Oak Ridge Natl Lab, Shull Wollan Ctr, Oak Ridge, TN 37831 USA
[13] Shanghai Jiao Tong Univ, Dept Phys & Astron, Key Lab Artificial Struct & Quantum Control, Shanghai 200240, Peoples R China
基金
美国国家科学基金会; 中国国家自然科学基金;
关键词
CHAIN; WAVE;
D O I
10.1103/PhysRevB.95.060412
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The perovskite Ba8CoNb6O24 comprises equilateral effective spin-1/2 Co2+ triangular layers separated by six nonmagnetic layers. Susceptibility, specific heat, and neutron scattering measurements combined with high-temperature series expansions and spin-wave calculations confirm that Ba8CoNb6O24 is basically a two-dimensional magnet with no detectable spin anisotropy and no long-range magnetic ordering down to 0.06 K. In other words, Ba8CoNb6O24 is very close to be a realization of the paradigmatic spin-1/2 triangular Heisenberg model, which is not expected to exhibit symmetry breaking at finite temperatures according to the Mermin and Wagner theorem.
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页数:5
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