The occurrence and distribution of pharmaceutical compounds in the effluents of a major sewage treatment plant in Northern Taiwan and the receiving coastal waters

被引:98
作者
Fang, Tien-Hsi [1 ]
Nan, Fan-Hua [2 ]
Chin, Tzong-Shean [3 ]
Feng, Hui-Min [1 ]
机构
[1] Natl Taiwan Ocean Univ, Dept Marine Environm Informat, Keelung 202, Taiwan
[2] Natl Taiwan Ocean Univ, Dept Aquaculture, Keelung 202, Taiwan
[3] Natl Chiayi Univ, Dept Aquat Biosci, Chiayi 500, Taiwan
关键词
Pharmaceutical residual; Sewage treatment plant; Ocean outfall; Environment risk quotient; PERSONAL CARE PRODUCTS; ENVIRONMENTAL RISK-ASSESSMENT; SOLID-PHASE EXTRACTION; MUNICIPAL WASTE-WATER; CLOFIBRIC ACID; TRACE-METALS; LIQUID-CHROMATOGRAPHY; ACTIVE COMPOUNDS; TANSHUI ESTUARY; DICLOFENAC;
D O I
10.1016/j.marpolbul.2012.04.008
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The pharmaceutical residues in waste water from the largest sewage treatment plant (SIP) in Northern Taiwan and in seawater around the effluent discharged area were determined. An environmental risk assessment for the marine environment was conducted based on the environment risk quotient (ERQ). The concentrations of the analyzed compounds in SIP influent and effluent were generally higher than those found in coastal seawater. Relatively higher values were found at the estuarine mouth and the discharged area, suggesting that the SIP effluent is a point source. The removal efficiency and half life of the analyzed compounds were 6.3-46.8% and 3-18 days, respectively. The ERQ value theoretical calculation was generally greater than 1. However, when the measured concentrations replaced the predicated concentrations, the ERQ values were considerably lower than 1. Therefore, our results call for a re-evaluation of the risks posed by pharmaceuticals to coastal marine ecosystems in Northern Taiwan. (C) 2012 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1435 / 1444
页数:10
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